Balazy M, Kaminski P M, Mao K, Tan J, Wolin M S
Departments of Pharmacology and Physiology, New York Medical College, Valhalla, New York 10595, USA.
J Biol Chem. 1998 Nov 27;273(48):32009-15. doi: 10.1074/jbc.273.48.32009.
Peroxynitrite (ONOO-) has been shown in studies on vascular relaxation and guanylate cyclase activation to react with glutathione (GSH), generating an intermediate product that promotes a time-dependent production of nitric oxide (NO). In this study, reactions of ONOO- with GSH produced a new substance, which was characterized by liquid chromatography, ultraviolet spectroscopy, and electrospray tandem mass spectrometry. The mass spectrometric data provided evidence that the product of this reaction was S-nitroglutathione (GSNO2) and that S-nitrosoglutathione (GSNO) was not a detectable product of this reaction. Further evidence was obtained by comparison of the spectral and chromatographic properties with synthetic standards prepared by reaction of GSH with nitrosonium or nitronium borofluorates. Both the synthetic and ONOO-/GSH-derived GSNO2 generated a protonated ion, GSNO2H+, at m/z 353, which was unusually resistant to decomposition under collision activation, and no fragmentation was observed at collision energy of 25 eV. In contrast, an ion at m/z 337 (GSNOH+), generated from the synthetic GSNO, readily fragmented with the abundant loss of NO at 9 eV. Reactions of ONOO- with GSH resulted in the generation of NO, which was detected by the head space/NO-chemiluminescence analyzer method. The generation of NO was inhibited by the presence of glucose and/or CO2 in the buffers employed. Synthetic GSNO2 spontaneously generated NO in a manner that was not significantly altered by glucose or CO2. Thus, ONOO- reacts with GSH to form GSNO2, and GSNO2 decomposes in a manner that generates NO.
过氧亚硝酸盐(ONOO-)在血管舒张和鸟苷酸环化酶激活的研究中已表明,它能与谷胱甘肽(GSH)反应,生成一种促进一氧化氮(NO)随时间产生的中间产物。在本研究中,ONOO-与GSH的反应产生了一种新物质,通过液相色谱、紫外光谱和电喷雾串联质谱对其进行了表征。质谱数据提供了证据,表明该反应的产物是S-硝基谷胱甘肽(GSNO2),且S-亚硝基谷胱甘肽(GSNO)不是该反应可检测到的产物。通过将光谱和色谱特性与由GSH与亚硝基或氟硼酸硝反应制备的合成标准品进行比较,获得了进一步的证据。合成的和由ONOO-/GSH衍生的GSNO2均在m/z 353处产生质子化离子GSNO2H+,该离子在碰撞激活下异常抗分解,在25 eV的碰撞能量下未观察到碎片化。相比之下,由合成的GSNO产生的m/z 337(GSNOH+)离子在9 eV时很容易碎片化,大量损失NO。ONOO-与GSH的反应导致NO的产生,通过顶空/NO化学发光分析仪方法检测到了NO的产生。在所使用的缓冲液中存在葡萄糖和/或CO2会抑制NO的产生。合成的GSNO2以一种不受葡萄糖或CO2显著影响的方式自发产生NO。因此,ONOO-与GSH反应形成GSNO2,且GSNO2以产生NO的方式分解。