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中纬度地区对流层溴氧化物的差分光学吸收光谱测量。

DOAS measurements of tropospheric bromine oxide in mid-latitudes.

作者信息

Hebestreit K, Stutz J, Rosen D, Matveiv V, Peleg M, Luria M, Platt U

机构信息

K. Hebestreit, J. Stutz, U. Platt, Institut fur Umweltphysik, Ruprecht-Karls-Universitat Heidelberg, Im Neuenheimer Feld 366, D-69120 Heidelberg, Germany. D. Rosen, V. Matveiv, M. Peleg, M. Luria, Environmental Science, School of Applie.

出版信息

Science. 1999 Jan 1;283(5398):55-7. doi: 10.1126/science.283.5398.55.

DOI:10.1126/science.283.5398.55
PMID:9872738
Abstract

Episodes of elevated bromine oxide (BrO) concentration are known to occur at high latitudes in the Arctic boundary layer and to lead to catalytic destruction of ozone at those latitudes; these events have not been observed at lower latitudes. With the use of differential optical absorption spectroscopy (DOAS), locally high BrO concentrations were observed at mid-latitudes at the Dead Sea, Israel, during spring 1997. Mixing ratios peaked daily at around 80 parts per trillion around noon and were correlated with low boundary-layer ozone mixing ratios.

摘要

已知在北极边界层的高纬度地区会出现溴氧化物(BrO)浓度升高的情况,并导致这些纬度地区的臭氧发生催化破坏;而在低纬度地区尚未观察到此类事件。利用差分光学吸收光谱法(DOAS),于1997年春季在以色列死海的中纬度地区观测到了局部高浓度的BrO。混合比在中午左右每日达到峰值,约为万亿分之80,并与低边界层臭氧混合比相关。

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