Zhitenev NB, Brodsky M, Ashoori RC, Pfeiffer LN, West KW
Department of Physics and Center for Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, MA 02139, USA. Bell Laboratories, Lucent Technologies, Murray Hill, NJ 07974, USA.
Science. 1999 Jul 30;285(5428):715-8. doi: 10.1126/science.285.5428.715.
Single-electron capacitance spectroscopy precisely measures the energies required to add individual electrons to a quantum dot. The spatial extent of electronic wave functions is probed by investigating the dependence of these energies on changes in the dot confining potential. For low electron densities, electrons occupy distinct spatial sites localized within the dot. At higher densities, the electrons become delocalized, and all wave functions are spread over the full dot area. Near the delocalization transition, the last remaining localized states exist at the perimeter of the dot. Unexpectedly, these electrons appear to bind with electrons in the dot center.
单电子电容光谱法精确测量向量子点逐个添加电子所需的能量。通过研究这些能量对量子点限制势变化的依赖性,来探测电子波函数的空间范围。对于低电子密度,电子占据量子点内局域化的不同空间位置。在较高密度时,电子变得离域,所有波函数扩展到整个量子点区域。在离域转变附近,最后剩余的局域态存在于量子点的周边。出乎意料的是,这些电子似乎与量子点中心的电子结合在一起。