Karrai Khaled, Warburton Richard J, Schulhauser Christian, Högele Alexander, Urbaszek Bernhard, McGhee Ewan J, Govorov Alexander O, Garcia Jorge M, Gerardot Brian D, Petroff Pierre M
Center for NanoScience and Sektion Physik, Ludwig-Maximilians-Universität, Geschwister-Scholl-Platz 1, 80539 München, Germany.
Nature. 2004 Jan 8;427(6970):135-8. doi: 10.1038/nature02109.
The self-assembly of semiconductor quantum dots has opened up new opportunities in photonics. Quantum dots are usually described as 'artificial atoms', because electron and hole confinement gives rise to discrete energy levels. This picture can be justified from the shell structure observed as a quantum dot is filled either with excitons (bound electron-hole pairs) or with electrons. The discrete energy levels have been most spectacularly exploited in single photon sources that use a single quantum dot as emitter. At low temperatures, the artificial atom picture is strengthened by the long coherence times of excitons in quantum dots, motivating the application of quantum dots in quantum optics and quantum information processing. In this context, excitons in quantum dots have already been manipulated coherently. We show here that quantum dots can also possess electronic states that go far beyond the artificial atom model. These states are a coherent hybridization of localized quantum dot states and extended continuum states: they have no analogue in atomic physics. The states are generated by the emission of a photon from a quantum dot. We show how a new version of the Anderson model that describes interactions between localized and extended states can account for the observed hybridization.
半导体量子点的自组装为光子学带来了新机遇。量子点通常被描述为“人造原子”,因为电子和空穴的限制产生了离散的能级。当量子点被激子(束缚的电子 - 空穴对)或电子填充时,从观察到的壳层结构可以证明这一图景的合理性。离散能级在以单个量子点作为发射器的单光子源中得到了最为显著的利用。在低温下,量子点中激子的长相干时间强化了人造原子的图景,推动了量子点在量子光学和量子信息处理中的应用。在这种背景下,量子点中的激子已经能够被相干地操控。我们在此表明,量子点还可以拥有远远超出人造原子模型的电子态。这些态是局域化量子点态和扩展连续态的相干杂化:它们在原子物理学中没有类似物。这些态是由量子点发射光子产生的。我们展示了一个描述局域态和扩展态之间相互作用的新版本安德森模型如何能够解释所观察到的杂化现象。