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通过超快X射线衍射检测非热熔化

Detection of nonthermal melting by ultrafast X-ray diffraction.

作者信息

Siders C W, Cavalleri A, Sokolowski-Tinten K, Tóth C, Guo T, Kammler M, Horn von Hoegen M, Wilson K R, von der Linde D, Barty C P

机构信息

Department of Chemistry and Biochemistry, Institute for Nonlinear Science, University of California, San Diego, La Jolla, CA 92093-0339, USA.

出版信息

Science. 1999 Nov 12;286(5443):1340-2. doi: 10.1126/science.286.5443.1340.

Abstract

Using ultrafast, time-resolved, 1.54 angstrom x-ray diffraction, thermal and ultrafast nonthermal melting of germanium, involving passage through nonequilibrium extreme states of matter, was observed. Such ultrafast, optical-pump, x-ray diffraction probe measurements provide a way to study many other transient processes in physics, chemistry, and biology, including direct observation of the atomic motion by which many solid-state processes and chemical and biochemical reactions take place.

摘要

利用超快、时间分辨的1.54埃X射线衍射,观察到锗的热熔化和超快非热熔化,其中涉及物质的非平衡极端状态。这种超快的光泵浦-X射线衍射探针测量提供了一种研究物理、化学和生物学中许多其他瞬态过程的方法,包括直接观察许多固态过程以及化学和生化反应发生时的原子运动。

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