Bayer M, Stern O, Hawrylak P, Fafard S, Forchel A
Technische Physik, Universitat Wurzburg, Germany.
Nature. 2000 Jun 22;405(6789):923-6. doi: 10.1038/35016020.
Quantum dots or 'artificial atoms' are of fundamental and technological interest--for example, quantum dots may form the basis of new generations of lasers. The emission in quantum-dot lasers originates from the recombination of excitonic complexes, so it is important to understand the dot's internal electronic structure (and of fundamental interest to compare this to real atomic structure). Here we investigate artificial electronic structure by injecting optically a controlled number of electrons and holes into an isolated single quantum dot. The charge carriers form complexes that are artificial analogues of hydrogen, helium, lithium, beryllium, boron and carbon excitonic atoms. We observe that electrons and holes occupy the confined electronic shells in characteristic numbers according to the Pauli exclusion principle. In each degenerate shell, collective condensation of the electrons and holes into coherent many-exciton ground states takes place; this phenomenon results from hidden symmetries (the analogue of Hund's rules for real atoms) in the energy function that describes the multi-particle system. Breaking of the hidden symmetries leads to unusual quantum interferences in emission involving excited states.
量子点或“人造原子”在基础研究和技术应用方面都备受关注——例如,量子点可能构成新一代激光器的基础。量子点激光器的发光源于激子复合体的复合,因此了解量子点的内部电子结构非常重要(并且将其与真实原子结构进行比较具有重要的基础研究意义)。在这里,我们通过向一个孤立的单量子点中光学注入可控数量的电子和空穴来研究人造电子结构。电荷载流子形成的复合体是氢、氦、锂、铍、硼和碳激子原子的人造类似物。我们观察到,根据泡利不相容原理,电子和空穴以特定数量占据受限的电子壳层。在每个简并壳层中,电子和空穴会集体凝聚成相干的多激子基态;这种现象源于描述多粒子系统的能量函数中的隐藏对称性(类似于真实原子的洪德规则)。隐藏对称性的破坏会导致涉及激发态的发射中出现异常的量子干涉。