用于关键有机化合物氢化反应的单步、高活性和高选择性纳米颗粒催化剂我们衷心感谢英国工程与自然科学研究委员会（EPSRC）（通过向J.M.T.提供的滚动资助以及向B.F.G.J.颁发的奖项）、剑桥海外信托基金（斯伦贝谢研究）和帝国化学工业公司（为T.K.提供资助）的支持，以及剑桥纽纳姆学院授予S.H.的研究奖学金。 - Suppr

Single-Step, Highly Active, and Highly Selective Nanoparticle Catalysts for the Hydrogenation of Key Organic Compounds We gratefully acknowledge the support (by a rolling grant to J.M.T. and an award to B.F.G.J.) of EPSRC (UK), of the Cambridge Overseas Trust (Schlumberger research), and ICI (for T.K.), and the award of a research fellowship (for S.H.) from Newnham College, Cambridge.

作者信息

Raja Robert, Khimyak Tetyana, Thomas John Meurig, Hermans Sophie, Johnson Brian F. G.

机构信息

The Royal Institution of Great Britain Davy Faraday Research Laboratory 21 Albemarle Street, London W1S 4BS (UK).

出版信息

Angew Chem Int Ed Engl. 2001 Dec 17;40(24):4638-4642. doi: 10.1002/1521-3773(20011217)40:24<4638::aid-anie4638>3.0.co;2-w.

DOI:10.1002/1521-3773(20011217)40:24<4638::aid-anie4638>3.0.co;2-w

PMID:12404371

Abstract

摘要

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Single-Step, Highly Active, and Highly Selective Nanoparticle Catalysts for the Hydrogenation of Key Organic Compounds We gratefully acknowledge the support (by a rolling grant to J.M.T. and an award to B.F.G.J.) of EPSRC (UK), of the Cambridge Overseas Trust (Schlumberger research), and ICI (for T.K.), and the award of a research fellowship (for S.H.) from Newnham College, Cambridge.用于关键有机化合物氢化反应的单步、高活性和高选择性纳米颗粒催化剂我们衷心感谢英国工程与自然科学研究委员会（EPSRC）（通过向J.M.T.提供的滚动资助以及向B.F.G.J.颁发的奖项）、剑桥海外信托基金（斯伦贝谢研究）和帝国化学工业公司（为T.K.提供资助）的支持，以及剑桥纽纳姆学院授予S.H.的研究奖学金。

Angew Chem Int Ed Engl. 2001 Dec 17;40(24):4638-4642. doi: 10.1002/1521-3773(20011217)40:24<4638::aid-anie4638>3.0.co;2-w.

Solvent-Free, Low-Temperature, Selective Hydrogenation of Polyenes using a Bimetallic Nanoparticle Ru-Sn Catalyst We thank Dr. R. G. Bell for assistance with the computer graphics, Drs. P. A. Midgeley, V. Keast, and M. Weyland for help with STEM, and gratefully acknowledge the support (via a rolling grant to J.M.T. and an award to B.F.G.J.) of EPSRC and the award of a research fellowship (for G.S.) from the Leverhulme Foundation and a Marie Curie Fellowship within the TMR Programme of the European Commission (for S.H.).使用双金属纳米颗粒Ru-Sn催化剂对多烯进行无溶剂、低温选择性氢化我们感谢R.G. Bell博士在计算机图形方面提供的帮助，感谢P.A. Midgeley博士、V. Keast博士和M. Weyland博士在扫描透射电子显微镜方面提供的帮助，并衷心感谢工程和物理科学研究委员会的支持（通过向J.M.T.提供的滚动资助以及向B.F.G.J.颁发的奖项），以及Leverhulme基金会授予的研究奖学金（给G.S.）和欧盟委员会TMR计划内的玛丽·居里奖学金（给S.H.）。

Angew Chem Int Ed Engl. 2001 Apr 1;40(7):1211-1215.

Designing a Molecular Sieve Catalyst for the Aerial Oxidation of n-Hexane to Adipic Acid We gratefully acknowledge helpful discussions with Dr. R. G. Bell and Prof. C. R. A. Catlow, the support (via a rolling grant to J.M.T.) of the EPSRC, and the award of a research fellowship (for G.S.) from the Leverhulme Foundation.设计用于将正己烷气相氧化为己二酸的分子筛催化剂我们衷心感谢与R.G.贝尔博士和C.R.A.卡特洛教授进行的有益讨论，感谢工程和物理科学研究委员会（通过向J.M.T.提供的滚动资助）的支持，以及利华休姆基金会授予（给G.S.）的研究奖学金。

Angew Chem Int Ed Engl. 2000 Jul 3;39(13):2313-2316. doi: 10.1002/1521-3773(20000703)39:13<2313::aid-anie2313>3.0.co;2-z.

Stereocontrolled Total Synthesis of (+)-Altohyrtin A/Spongistatin 1 Financial support was provided by the EPSRC (GR/L41646), Cambridge Commonwealth Trust (Scholarship to M.J.C.), EC (Marie Curie Postdoctoral Fellowship to J.L.A.), DFG (Postdoctoral Fellowship to T.T.), NSERC-Canada (Postdoctoral Fellowship to R.M.O.), Churchill College (Research Fellowship to D.J.W.), Kingapos;s College and Sims Fund, Cambridge (Scholarship to D.Y.K.C.). We also thank Merck and AstraZeneca Pharmaceuticals for generous support, and Dr. Anne Butlin (AZ) and Dr. Nick Bampos (Cambridge) for valuable assistance.（+）-Altohyrtin A/海绵抑素1的立体控制全合成本研究得到了英国工程与自然科学研究委员会（GR/L41646）、剑桥联邦信托基金（授予M.J.C.的奖学金）、欧盟（授予J.L.A.的玛丽·居里博士后奖学金）、德国研究基金会（授予T.T.的博士后奖学金）、加拿大自然科学与工程研究理事会（授予R.M.O.的博士后奖学金）、丘吉尔学院（授予D.J.W.的研究奖学金）、国王学院和剑桥西姆斯基金（授予D.Y.K.C.的奖学金）的资金支持。我们还要感谢默克公司和阿斯利康制药公司的慷慨支持，以及安妮·巴特林博士（阿斯利康）和尼克·班波斯博士（剑桥）提供的宝贵帮助。

Angew Chem Int Ed Engl. 2001 Nov 5;40(21):4055-4060.

Direct Comparison of Hydrogenation Catalysis by Intact versus Fragmented Triruthenium Clusters D.B. acknowledges financial support from the ORS Award Scheme. S.B.D. is grateful to the EPSRC, the JREI Scheme, and Bruker UK for financial support. P.J.D. thanks the Royal Society for a University Research Fellowship. Discussions with Prof. R. Eisenberg (NATO support), Prof. B. F. G. Johnson, Prof. R. N. Perutz, and Dr. R. J. Mawby are gratefully acknowledged.完整与碎片化三钌簇催化氢化反应的直接比较 D.B. 感谢ORS奖励计划提供的资金支持。S.B.D. 感谢工程和物理科学研究委员会、联合研究设备倡议计划以及英国布鲁克公司提供的资金支持。P.J.D. 感谢皇家学会授予大学研究奖学金。感谢与R. 艾森伯格教授（北约支持）、B.F.G. 约翰逊教授、R.N. 佩鲁茨教授以及R.J. 莫比博士的讨论。

Angew Chem Int Ed Engl. 2001 Oct 15;40(20):3874-3877.

Formation of Aryl- and Benzylboronate Esters by Rhodium-Catalyzed C-H Bond Functionalization with Pinacolborane The EPSRC is gratefully acknowledged for financial support (T.B.M. and J.A.K.H.) and for a Senior Fellowship (J.A.K.H.). Dr. Shimada thanks the Science and Technology Agency of Japan for a fellowship, and Dr. M. Tanaka for granting sabbatical leave, making possible his stay in Durham. We thank Prof. M. Srebnik for advice on the purification of HBpin.通过铑催化的与频哪醇硼烷的C-H键官能化反应形成芳基硼酸酯和苄基硼酸酯感谢工程和物理科学研究委员会（EPSRC）提供资金支持（T.B.M.和J.A.K.H.）以及高级研究奖学金（J.A.K.H.）。岛田博士感谢日本科学技术厅提供奖学金，感谢田中博士批准其休假，使其能够在达勒姆停留。我们感谢M. Srebnik教授在频哪醇硼烷纯化方面提供的建议。

Angew Chem Int Ed Engl. 2001 Jun 1;40(11):2168-2171.

Consecutive Three- and Four-Component Coupling Reactions with Anions Generated from a Butane Diacetal Desymmetrized Glycolic Acid Derivative We gratefully acknowledge financial support from the EPSRC (to D.J.D.), the EU (Marie Curie Fellowship to F.R.), and the Novartis Research Fellowship (to S.V.L.). We are also indebted to Dr. John E. Davis for the X-ray crystal structure determinations.由丁烷二缩醛去对称化乙醇酸衍生物产生的阴离子的连续三组分和四组分偶联反应我们衷心感谢EPSRC（给D.J.D.）、欧盟（给F.R.的玛丽·居里奖学金）和诺华研究奖学金（给S.V.L.）提供的资金支持。我们还感谢John E. Davis博士进行的X射线晶体结构测定。

Angew Chem Int Ed Engl. 2001 Dec 17;40(24):4763-4765. doi: 10.1002/1521-3773(20011217)40:24<4763::aid-anie4763>3.0.co;2-d.

Resolution and Kinetic Stability of a Chiral Supramolecular Assembly Made of Labile Components Coordination Number Incommensurate Cluster Formation, Part 18. Financial support of this work was provided by NSF CHE-9709621 and by NSF and NATO-NSF exchange grants INT-9603212 and SRG 951516, respectively. We thank the Alexander-von-Humboldt Foundation for a Fellowship to A.T., and a Humboldt Research Award for Senior U.S. Scientists to K.R., and the Miller Foundation for a fellowship to M.Z. The authors gratefully acknowledge the assistance of Dr. F. J. Hollander and Dr. D. L. Caulder in selecting and mounting a suitable single crystal, and Prof. Julie A. Leary, Dr. Ulla N. Andersen, and J. J. Miranda for measuring mass spectra. Part 17: M. Ziegler, J. J. Miranda, U. N. Andersen, D. W. Johnson, J. A. Leary, K. N. Raymond, Angew. Chem., in press.由不稳定组分构成的手性超分子组装体的分辨率和动力学稳定性：配位数不匹配的簇形成，第18部分。本研究得到了美国国家科学基金会（NSF）CHE - 9709621项目以及NSF和北约 - NSF交流基金INT - 9603212和SRG 951516的资助。我们感谢亚历山大·冯·洪堡基金会授予A.T.的奖学金、授予K.R.的洪堡资深美国科学家研究奖，以及米勒基金会授予M.Z.的奖学金。作者们衷心感谢F. J. 霍兰德博士和D. L. 考尔德博士在挑选和安装合适单晶方面提供的帮助，以及朱莉·A. 利里教授、乌拉·N. 安德森博士和J. J. 米兰达在测量质谱方面提供的帮助。第17部分：M. 齐格勒、J. J. 米兰达、U. N. 安德森、D. W. 约翰逊、J. A. 利里、K. N. 雷蒙德，《德国应用化学》，即将发表。

Angew Chem Int Ed Engl. 2001 Jan 5;40(1):157-160.

Toward Fully Synthetic Homogeneous Glycoproteins: A High Mannose Core Containing Glycopeptide Carrying Full H-Type 2 Human Blood Group Specificity This work was supported by the National Institutes of Health (Grant nos.: HL-25848 and CA-28824 (to S.J.D.), and CA-710506 (to K.O.L.)). Postdoctoral fellowship support is gratefully acknowledged by Z.-G.W. (US Army breast cancer grant no.: DAMD17-97-1-7119) and M.V. (NIH grant no.: CA-62948-04). We gratefully acknowledge Dr. George Sukenick of the Sloan-Kettering Institute's NMR core facility for mass spectral and NMR spectroscopic analyses (SKI core grant no.: CA-08748).

Angew Chem Int Ed Engl. 2001 May 4;40(9):1728-1732.

Stabilization of a Reactive Cationic Species by Supramolecular Encapsulation Coordination Number Incommensurate Cluster Formation, Part 15. This research was supported by NSF grant CHE-9709621. We gratefully acknowledge Prof. Julie A. Leary and Dr. Ulla Andersen for their assistance with mass spectrometry. We also thank the Miller Foundation for a postdoctoral fellowship to M.Z. and the NIH for a postdoctoral fellowship to J.L.B. Part 14: J. Xide, K. N. Raymond, Angew. Chem. 2000, 112, 2857-2859; Angew. Chem. Int. Ed. 2000, 39, 2745-2747.通过超分子包封稳定反应性阳离子物种：配位数不匹配簇的形成，第15部分。本研究得到美国国家科学基金会（NSF）CHE - 9709621号资助。我们非常感谢朱莉·A·利里教授和乌拉·安德森博士在质谱分析方面提供的帮助。我们还要感谢米勒基金会为M.Z.提供博士后奖学金，以及美国国立卫生研究院（NIH）为J.L.B.提供博士后奖学金。第14部分：J. 西德，K. N. 雷蒙德，《德国应用化学》，2000年，112卷，2857 - 2859页；《德国应用化学》国际版，2000年，39卷，2745 - 2747页。

Angew Chem Int Ed Engl. 2000 Nov 17;39(22):4119-4121. doi: 10.1002/1521-3773(20001117)39:22<4119::aid-anie4119>3.0.co;2-1.

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