Berthier Ludovic
Theoretical Physics, University of Oxford, 1 Keble Road, Oxford OX1 3NP, United Kingdom.
Phys Rev E Stat Nonlin Soft Matter Phys. 2004 Feb;69(2 Pt 1):020201. doi: 10.1103/PhysRevE.69.020201. Epub 2004 Feb 27.
We numerically obtain a quantitative demonstration that development of spatial correlations of mobility as temperature is lowered is responsible for the "decoupling" of transport properties of supercooled liquids. This result further demonstrates the necessity of a spatial description of the glass formation and therefore seriously challenges a number of popular alternative theoretical descriptions.
我们通过数值计算得到了一个定量的论证,即随着温度降低,迁移率的空间相关性的发展是过冷液体输运性质“解耦”的原因。这一结果进一步证明了对玻璃形成进行空间描述的必要性,因此严重挑战了一些流行的替代理论描述。