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美国西南部干旱地区扬尘的沉降与清除:测量结果与模型结果

Deposition and removal of fugitive dust in the arid southwestern United States: measurements and model results.

作者信息

Etyemezian Vic, Ahonen Sean, Nikolic Djordje, Gillies John, Kuhns Hampden, Gillette Dale, Veranth John

机构信息

Division of Atmospheric Sciences, Desert Research Institute, Las Vegas, Nevada 89119, USA.

出版信息

J Air Waste Manag Assoc. 2004 Sep;54(9):1099-111. doi: 10.1080/10473289.2004.10470977.

Abstract

This work was motivated by the need to better reconcile emission factors for fugitive dust with the amount of geologic material found on ambient filter samples. The deposition of particulate matter with aerodynamic diameter less than or equal to 10 microm (PM10), generated by travel over an unpaved road, over the first 100 m of transport downwind of the road was examined at Ft. Bliss, near El Paso, TX. The field conditions, typical for warm days in the arid southwestern United States, represented sparsely vegetated terrain under neutral to unstable atmospheric conditions. Emission fluxes of PM10 dust were obtained from towers downwind of the unpaved road at 7, 50, and 100 m. The horizontal flux measurements at the 7 m and 100 m towers indicated that PM10 deposition to the vegetation and ground was too small to measure. The data indicated, with 95% confidence, that the loss of PM10 between the source of emission at the unpaved road, represented by the 7 m tower, and a point 100 m downwind was less than 9.5%. A Gaussian model was used to simulate the plume. Values of the vertical standard deviation sigma(z) and the deposition velocity Vd were similar to the U.S. Environmental Protection Agency (EPA) ISC3 model. For the field conditions, the model predicted that removal of PM10 unpaved road dust by deposition over the distance between the point of emission and 100 m downwind would be less than 5%. However, the model results also indicated that particles larger than 10 microm (aerodynamic diameter) would deposit more appreciably. The model was consistent with changes observed in size distributions between 7 m and 100 m downwind, which were measured with optical particle counters. The Gaussian model predictions were also compared with another study conducted over rough terrain and stable atmospheric conditions. Under such conditions, measured PM10 removal rates over 95 m of downwind transport were reported to be between 86% and 89%, whereas the Gaussian model predicted only a 30% removal. One explanation for the large discrepancy between measurements and model results was the possibility that under the conditions of the study, the dust plume was comparable in vertical extent to the roughness elements, thereby violating one of the model assumptions. Results of the field study reported here and the previous work over rough terrain bound the extent of particle deposition expected to occur under most unpaved road emission scenarios.

摘要

开展这项工作的动机是,需要更好地使扬尘排放因子与环境过滤器样本中发现的地质物质数量相协调。在德克萨斯州埃尔帕索附近的布利斯堡,对在未铺砌道路上行驶产生的空气动力学直径小于或等于10微米的颗粒物(PM10)在道路下风方向前100米处的沉积情况进行了研究。该野外条件是美国西南部干旱地区温暖日子的典型情况,代表了中性至不稳定大气条件下植被稀少的地形。在未铺砌道路下风方向7米、50米和100米处的塔上获取了PM10粉尘的排放通量。7米和100米塔处的水平通量测量表明,PM10在植被和地面上的沉积量太小,无法测量。数据表明,在95%的置信度下,以7米塔为代表的未铺砌道路排放源与下风方向100米处之间PM10的损失小于9.5%。使用高斯模型来模拟烟羽。垂直标准差sigma(z)和沉积速度Vd的值与美国环境保护局(EPA)的ISC3模型相似。对于野外条件,该模型预测,在排放点与下风方向100米之间的距离上,通过沉积去除未铺砌道路上的PM10粉尘量将小于5%。然而,模型结果还表明,空气动力学直径大于10微米的颗粒沉积会更明显。该模型与在7米和下风方向100米处用光学粒子计数器测量的粒径分布变化一致。高斯模型的预测结果还与另一项在粗糙地形和稳定大气条件下进行的研究进行了比较。在这种条件下,据报道,下风方向95米传输距离内测得的PM10去除率在86%至89%之间,而高斯模型仅预测去除率为30%。测量结果与模型结果之间存在巨大差异的一个解释是,在该研究条件下,粉尘烟羽在垂直范围上可能与粗糙度元素相当,从而违反了模型假设之一。此处报告的野外研究结果以及之前在粗糙地形上的工作界定了在大多数未铺砌道路排放情景下预期发生的颗粒沉积程度。

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