Wilflinger T, Lettner H, Hubmer A K, Hofmann W
Institute of Physics and Biophysics, University of Salzburg, Hellbrunnerstrasse 34, A-5020 Salzburg, Austria.
J Environ Radioact. 2005;83(1):75-89. doi: 10.1016/j.jenvrad.2005.02.014. Epub 2005 Apr 11.
In this study the runoff of (137)Cs, mainly originated from the Chernobyl fallout, from highly contaminated alpine regions in Salzburg (Austria) is discussed. Twenty-five water-samples and 25 sediment-samples were taken from creeks of different size to determine the runoff of dissolved (137)Cs and Cs-binding characteristics to different particle size classes in the sediments. The hypothesis, that specific activity of the sediments depended on particle size and the surface of the particle, was proved with some modifications. Caesium activity concentration in water showed a negative correlation with electrical conductivity, while no significant correlations were detectable with other variables (pH, temperature, and altitude). Enormous differences and the variations found in the (137)Cs-concentrations in water can be explained by the electrical conductivity without any dependency on the inventory of the catchment. The sediment samples analysed showed a negative correlation between specific activity [Bq/kg] and particle-diameter, mainly explained by (137)Cs-uptake proportional to the particle surface per mass.
本研究讨论了主要源自切尔诺贝利放射性尘埃的铯-137从奥地利萨尔茨堡高污染山区的径流情况。从不同大小的溪流中采集了25个水样和25个沉积物样本,以确定溶解态铯-137的径流以及沉积物中铯与不同粒径粒级的结合特性。沉积物比活度取决于粒径和颗粒表面这一假设在经过一些修正后得到了证实。水中铯活度浓度与电导率呈负相关,而与其他变量(pH值、温度和海拔)未检测到显著相关性。水中铯-137浓度的巨大差异和变化可以用电导率来解释,而与集水区的存量无关。分析的沉积物样本显示比活度[Bq/kg]与粒径之间呈负相关,这主要是由于铯-137的吸收与单位质量的颗粒表面成正比。