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单个分子的散粒噪声测量

Shot noise measurements on a single molecule.

作者信息

Djukic D, van Ruitenbeek J M

机构信息

Kamerlingh Onnes Laboratorium, Universiteit Leiden, Postbus 9504, NL-2300 RA Leiden, The Netherlands.

出版信息

Nano Lett. 2006 Apr;6(4):789-93. doi: 10.1021/nl060116e.

Abstract

We report measurements of shot noise in the current through a single D2 molecule. The molecular junctions were formed by means of the mechanically controllable break junction technique. The configuration of the D2 molecule bridging the gap between two Pt tips is verified by use of point contact spectroscopy. Maintaining the same junction shot noise measurements were performed and the observed quantum suppression shows that conductance is carried dominantly by a single, almost fully transparent conductance channel. This observation allows us to decide between conflicting model calculations for this system, and this may serve as a benchmark for further computations on molecular junctions.

摘要

我们报告了通过单个D2分子的电流中的散粒噪声测量结果。分子结是通过机械可控断裂结技术形成的。利用点接触光谱法验证了D2分子桥接两个铂尖端之间间隙的结构。在保持相同结的情况下进行了散粒噪声测量,观察到的量子抑制表明,电导主要由单个几乎完全透明的电导通道承载。这一观察结果使我们能够在该系统相互矛盾的模型计算之间做出决定,这可能为分子结的进一步计算提供一个基准。

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