Kordonis K, Sologubenko A V, Lorenz T, Cheong S-W, Freimuth A
II. Physikalisches Institut, Universität zu Köln, 50937 Köln, Germany.
Phys Rev Lett. 2006 Sep 15;97(11):115901. doi: 10.1103/PhysRevLett.97.115901. Epub 2006 Sep 13.
We have measured the thermal conductivity of the spin S=1 chain compound Y(2)BaNiO(5). Analyzing the anisotropy of the thermal transport allows us to identify a definite spin-mediated thermal conductivity kappa(s) along the chain direction. The calculated spin-related energy diffusion constant D(E)(T) shows a broad peak around 120 K. Close to room temperature, D(E)(T) approaches the theoretically predicted high-temperature value, while scattering of spin excitations by magnetic impurities seems to be the major limiting factor of kappa(s) at low temperature.