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Ultrafast Fano resonance between optical phonons and electron-hole pairs at the onset of quasiparticle generation in a semiconductor.

作者信息

Lee J D, Inoue J, Hase Muneaki

机构信息

International Center for Young Scientists, National Institute for Materials Science, Tsukuba 305-0044, Japan.

出版信息

Phys Rev Lett. 2006 Oct 13;97(15):157405. doi: 10.1103/PhysRevLett.97.157405. Epub 2006 Oct 11.

DOI:10.1103/PhysRevLett.97.157405
PMID:17155359
Abstract

Based on the many-body time-dependent approach applied to the ultrafast time region, we investigate the dynamics of creation of an optical phonon incorporating with the electron-hole continuum in a semiconductor. In the transient Fano resonance, due to an interference between those sharp (optical phonon) and continuum (electron-hole pair) quasiparticles, we find the robust destructive interference at birth of them, i.e., tau approximately 0 if the created phonon is coherent under the irradiation of ultrashort optical pulses. The origin is found to be the potential scattering of the electron-hole pair by the q=0 coherent phonon. This finding agrees well with the recent experiment.

摘要

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引用本文的文献

1
Ultrafast Spectroscopy of Fano-Like Resonance between Optical Phonon and Excitons in CdSe Quantum Dots: Dependence of Coherent Vibrational Wave-Packet Dynamics on Pump Fluence.CdSe量子点中光学声子与激子之间类Fano共振的超快光谱:相干振动波包动力学对泵浦通量的依赖性。
Nanomaterials (Basel). 2017 Nov 4;7(11):371. doi: 10.3390/nano7110371.