Yoshino S, Oohata G, Mizoguchi K
Department of Physical Science, Graduate School of Science, Osaka Prefecture University, 1-1 Gakuen-cho, Naka-ku, Sakai 599-8531, Japan.
Phys Rev Lett. 2015 Oct 9;115(15):157402. doi: 10.1103/PhysRevLett.115.157402. Epub 2015 Oct 7.
We report on dynamical interference between short-lived Rabi oscillations and long-lived coherent phonons in CuCl semiconductor microcavities resulting from the coupling between the two oscillations. The Fourier-transformed spectra of the time-domain signals obtained from semiconductor microcavities by using a pump-probe technique show that the intensity of the coherent longitudinal optical phonon of CuCl is enhanced by increasing that of the Rabi oscillation, which indicates that the coherent phonon is driven by the Rabi oscillation through the Fröhlich interaction. Moreover, as the Rabi oscillation frequency decreases upon crossing the phonon frequency, the spectral profile of the coherent phonon changes from a peak to a dip with an asymmetric structure. The continuous wavelet transformation reveals that these peak and dip structures originate from constructive and destructive interference between Rabi oscillations and coherent phonons, respectively. We demonstrate that the asymmetric spectral structures in relation to the frequency detuning are well reproduced by using a classical coupled oscillator model on the basis of dynamical Fano-like interference.
我们报道了在CuCl半导体微腔中,由短寿命拉比振荡和长寿命相干声子之间的耦合所导致的动态干涉。通过泵浦-探测技术从半导体微腔获得的时域信号的傅里叶变换光谱表明,通过增加拉比振荡的强度,CuCl的相干纵向光学声子的强度会增强,这表明相干声子是通过弗罗里希相互作用由拉比振荡驱动的。此外,当拉比振荡频率在穿过声子频率时降低,相干声子的光谱轮廓从一个峰变为具有不对称结构的谷。连续小波变换表明,这些峰和谷结构分别源于拉比振荡和相干声子之间的相长干涉和相消干涉。我们证明,基于动态类法诺干涉,使用经典耦合振荡器模型可以很好地再现与频率失谐相关的不对称光谱结构。