He J, Krenner H J, Pryor C, Zhang J P, Wu Y, Allen D G, Morris C M, Sherwin M S, Petroff P M
Materials Department, University of California, Santa Barbara, California 93106, USA.
Nano Lett. 2007 Mar;7(3):802-6. doi: 10.1021/nl070132r. Epub 2007 Feb 28.
Self-assembled quantum dots embedded in semiconductor heterostructures have proved to be a rich system for exploring the physics of three dimensionally confined charges and excitons. We present here a novel structure, which allows adjusting the level of confinement between 3D and 2D for electrons and holes, respectively. The quantum post consists of a quantum dot connected to a short quantum wire. The molecular beam epitaxy deposition of these self-assembled structures is discussed, and their structural and chemical compositions are presented. Their optical properties measured by photoluminescence are compared to an eight-band strain-dependent k.p model incorporating detailed structure and alloy composition. The calculations show electron delocalization in the quantum wire part of the quantum post and hole localization in the strain-induced regions at the ends of the quantum post. The quantum post offers the possibility of controlling the dipole moment in the structure and opens up new means for tuning the intra-subband transitions by controlling its dimensions.
嵌入半导体异质结构中的自组装量子点已被证明是探索三维受限电荷和激子物理的丰富系统。我们在此展示一种新颖的结构,它分别允许对电子和空穴在三维和二维之间的受限程度进行调节。量子柱由连接到短量子线的量子点组成。讨论了这些自组装结构的分子束外延生长,并给出了它们的结构和化学成分。将通过光致发光测量的它们的光学性质与包含详细结构和合金成分的八能带应变相关k.p模型进行了比较。计算表明,电子在量子柱的量子线部分离域,而空穴则定域在量子柱端部的应变诱导区域。量子柱提供了控制结构中偶极矩的可能性,并通过控制其尺寸开辟了调节子带内跃迁的新方法。