Kopp Angela, Ghosal Amit, Chakravarty Sudip
Department of Physics and Astronomy, University of California, Los Angeles, CA 90095, USA.
Proc Natl Acad Sci U S A. 2007 Apr 10;104(15):6123-7. doi: 10.1073/pnas.0701265104. Epub 2007 Apr 2.
The extreme variability of observables across the phase diagram of the cuprate high-temperature superconductors has remained a profound mystery, with no convincing explanation for the superconducting dome. Although much attention has been paid to the underdoped regime of the hole-doped cuprates because of its proximity to a complex Mott insulating phase, little attention has been paid to the overdoped regime. Experiments are beginning to reveal that the phenomenology of the overdoped regime is just as puzzling. For example, the electrons appear to form a Landau Fermi liquid, but this interpretation is problematic; any trace of Mott phenomena, as signified by incommensurate antiferromagnetic fluctuations, is absent, and the uniform spin susceptibility shows a ferromagnetic upturn. Here, we show and justify that many of these puzzles can be resolved if we assume that competing ferromagnetic fluctuations are simultaneously present with superconductivity, and the termination of the superconducting dome in the overdoped regime marks a quantum critical point beyond which there should be a genuine ferromagnetic phase at zero temperature. We propose experiments and make predictions to test our theory and suggest that an effort must be mounted to elucidate the nature of the overdoped regime, if the problem of high-temperature superconductivity is to be solved. Our approach places competing order as the root of the complexity of the cuprate phase diagram.
铜酸盐高温超导体相图中可观测值的极端变异性一直是个深奥的谜团,对于超导穹顶没有令人信服的解释。尽管由于空穴掺杂铜酸盐的欠掺杂区域接近复杂的莫特绝缘相而备受关注,但对过掺杂区域却很少关注。实验开始揭示,过掺杂区域的现象学同样令人困惑。例如,电子似乎形成了朗道费米液体,但这种解释存在问题;不存在任何由非公度反铁磁涨落所表征的莫特现象痕迹,并且均匀自旋磁化率呈现出铁磁上升。在此,我们表明并论证,如果假设竞争的铁磁涨落与超导同时存在,那么许多这些谜题可以得到解决,并且过掺杂区域中超导穹顶的终止标志着一个量子临界点,超过该点在零温度下应该存在一个真正的铁磁相。我们提出实验并做出预测以检验我们的理论,并表明如果要解决高温超导问题,必须努力阐明过掺杂区域的性质。我们的方法将竞争序作为铜酸盐相图复杂性的根源。