Lal Rattan
Carbon Management and Sequestration Center, The Ohio State University, Columbus, OH 43210, USA.
Philos Trans R Soc Lond B Biol Sci. 2008 Feb 27;363(1492):815-30. doi: 10.1098/rstb.2007.2185.
Developing technologies to reduce the rate of increase of atmospheric concentration of carbon dioxide (CO2) from annual emissions of 8.6PgCyr-1 from energy, process industry, land-use conversion and soil cultivation is an important issue of the twenty-first century. Of the three options of reducing the global energy use, developing low or no-carbon fuel and sequestering emissions, this manuscript describes processes for carbon (CO2) sequestration and discusses abiotic and biotic technologies. Carbon sequestration implies transfer of atmospheric CO2 into other long-lived global pools including oceanic, pedologic, biotic and geological strata to reduce the net rate of increase in atmospheric CO2. Engineering techniques of CO2 injection in deep ocean, geological strata, old coal mines and oil wells, and saline aquifers along with mineral carbonation of CO2 constitute abiotic techniques. These techniques have a large potential of thousands of Pg, are expensive, have leakage risks and may be available for routine use by 2025 and beyond. In comparison, biotic techniques are natural and cost-effective processes, have numerous ancillary benefits, are immediately applicable but have finite sink capacity. Biotic and abiotic C sequestration options have specific nitches, are complementary, and have potential to mitigate the climate change risks.
通过技术手段降低能源、加工工业、土地利用变化和土壤耕作每年排放8.6PgC碳所导致的大气二氧化碳(CO₂)浓度增长率,是21世纪的一个重要问题。在减少全球能源使用、开发低碳或无碳燃料以及封存排放这三种选择中,本文描述了碳(CO₂)封存的过程,并讨论了非生物和生物技术。碳封存意味着将大气中的CO₂转移到其他长期存在的全球库中,包括海洋、土壤、生物和地质层,以降低大气CO₂的净增长率。向深海、地质层、旧煤矿和油井以及盐水层注入CO₂的工程技术,以及CO₂的矿物碳酸化,构成了非生物技术。这些技术具有数千Pg的巨大潜力,成本高昂,存在泄漏风险,可能在2025年及以后用于常规应用。相比之下,生物技术是自然且具有成本效益的过程,有许多附带益处,可立即应用,但汇容量有限。生物和非生物碳封存选择具有特定的适用范围,相互补充,有潜力降低气候变化风险。