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生物质露天焚烧对环境空气中多氯二苯并对二噁英和二苯并呋喃水平的影响

Significance of biomass open burning on the levels of polychlorinated dibenzo-p-dioxins and dibenzofurans in the ambient air.

作者信息

Shih Shun-I, Lee Wen-Jhy, Lin Long-Full, Huang Jiao-Yan, Su Jen-Wei, Chang-Chien Guo-Ping

机构信息

Department of Environmental Engineering, Kun Shan University, Yung-Kang, Taiwan.

出版信息

J Hazard Mater. 2008 May 1;153(1-2):276-84. doi: 10.1016/j.jhazmat.2007.08.048. Epub 2007 Aug 22.

DOI:10.1016/j.jhazmat.2007.08.048
PMID:17897777
Abstract

In southern Taiwan, two areas (L- and Y-) with/without biomass open burning were selected to compare the PCDD/F concentrations and their congener profiles in the ambient air. The results of this study indicate that biomass (rice straw) open burning exhibited a significant impact on the PCDD/F concentration level in the ambient air. During the biomass burning season, the total PCDD/F I-TEQ concentrations in the ambient air of L- and Y-areas were approximately 4 and 17 times higher than those without biomass open burning, respectively. When 10% mass fraction of rice straw was burned, the contribution fraction of biomass burning on annual total PCDD/F I-TEQ emission was 3.28 and 8.11% for KC County and for Taiwan, respectively; however, when the calculation was on a weekly basis, the contribution fraction of biomass burning on weekly total PCDD/F I-TEQ emission was 30.6 and 53.4% for KC County and for Taiwan, respectively. The results of this study imply that during the week of biomass burning, it appears to be the most significant source of total I-TEQ PCDD emission. The results of this research can be applied to the study of other agricultural areas.

摘要

在台湾南部,选择了两个有/无生物质露天焚烧的区域(L区和Y区),以比较环境空气中多氯二苯并对二恶英/多氯二苯并呋喃(PCDD/F)的浓度及其同系物分布。本研究结果表明,生物质(稻草)露天焚烧对环境空气中PCDD/F的浓度水平有显著影响。在生物质燃烧季节,L区和Y区环境空气中PCDD/F的总毒性当量(I-TEQ)浓度分别比无生物质露天焚烧时高出约4倍和17倍。当燃烧10%质量分数的稻草时,高雄县和台湾地区生物质燃烧对年度PCDD/F总I-TEQ排放的贡献率分别为3.28%和8.11%;然而,按周计算时,高雄县和台湾地区生物质燃烧对每周PCDD/F总I-TEQ排放的贡献率分别为30.6%和53.4%。本研究结果表明,在生物质燃烧的那一周,它似乎是I-TEQ总PCDD排放的最重要来源。本研究结果可应用于其他农业地区的研究。

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