Park Seungkyung, Beskok Ali
Aerospace Engineering Department, Old Dominion University, Norfolk, Virginia 23529, USA.
Anal Chem. 2008 Apr 15;80(8):2832-41. doi: 10.1021/ac7024859. Epub 2008 Mar 5.
Alternating current (ac) electrokinetic motion of colloidal particles suspended in an aqueous medium and subjected to a spatially nonuniform ac electric field are examined using a simple theoretical model that considers the relative magnitudes of dielectrophoresis, electrophoresis, ac-electroosmosis, and Brownian motion. Dominant electrokinetic forces are explained as a function of the electric field frequency, amplitude, and conductivity of the suspending medium for given material properties and geometry. Parametric experimental validations of the model are conducted utilizing interdigitated microelectrodes with polystyrene and gold particles and Clostridium sporogenes bacterial spores. The theoretical model provides quantitative descriptions of ac electrokinetic transport for the given target species in a wide spectrum of electric field amplitude and frequency and medium conductivity. The presented model can be used as an effective framework for design and optimization of ac electrokinetic devices.
使用一个简单的理论模型来研究悬浮在水性介质中并受到空间非均匀交流电场作用的胶体颗粒的交流(ac)电动运动,该模型考虑了介电泳、电泳、交流电渗和布朗运动的相对大小。对于给定的材料特性和几何形状,主要的电动作用力被解释为电场频率、幅度和悬浮介质电导率的函数。利用带有聚苯乙烯和金颗粒以及生孢梭菌芽孢的叉指微电极对该模型进行了参数实验验证。该理论模型对给定目标物种在很宽的电场幅度、频率和介质电导率范围内的交流电动输运提供了定量描述。所提出的模型可作为设计和优化交流电动装置的有效框架。