Suppr超能文献

由随机顺序吸附驱动的棘轮的精确稳态速度。

Exact steady-state velocity of ratchets driven by random sequential adsorption.

作者信息

D'Orsogna Maria R, Chou Tom, Antal Tibor

机构信息

Department of Mathematics, UCLA, Los Angeles, CA 90095-1555.

出版信息

J Phys A Math Gen. 2007 May 25;40(21):5575-5584. doi: 10.1088/1751-8113/40/21/009.

Abstract

We solve the problem of discrete translocation of a polymer through a pore, driven by the irreversible, random sequential adsorption of particles on one side of the pore. Although the kinetics of the wall motion and the deposition are coupled, we find the exact steady-state distribution for the gap between the wall and the nearest deposited particle. This result enables us to construct the mean translocation velocity demonstrating that translocation is faster when the adsorbing particles are smaller. Monte-Carlo simulations also show that smaller particles gives less dispersion in the ratcheted motion. We also define and compare the relative efficiencies of ratcheting by deposition of particles with different sizes and we describe an associated "zone-refinement" process.

摘要

我们解决了聚合物通过孔隙的离散易位问题,该过程由孔隙一侧颗粒的不可逆随机顺序吸附驱动。尽管壁运动和沉积的动力学是耦合的,但我们找到了壁与最近沉积颗粒之间间隙的精确稳态分布。这一结果使我们能够构建平均易位速度,表明当吸附颗粒较小时易位速度更快。蒙特卡罗模拟还表明,较小的颗粒在棘轮运动中的分散性较小。我们还定义并比较了不同尺寸颗粒沉积产生棘轮效应的相对效率,并描述了相关的“区域细化”过程。

相似文献

2
Irreversible adsorption of particles on heterogeneous surfaces.颗粒在异质表面上的不可逆吸附。
Adv Colloid Interface Sci. 2005 Dec 30;118(1-3):25-42. doi: 10.1016/j.cis.2005.03.003. Epub 2005 Jun 14.
4
Effects of an attractive wall on the translocation of polymer under driving.在驱动力作用下聚合物的输运中壁面吸引力的影响。
J Phys Condens Matter. 2012 Aug 15;24(32):325104, 1-8. doi: 10.1088/0953-8984/24/32/325104. Epub 2012 Jun 26.
5
Random sequential adsorption on mobile patches.随机顺序吸附在可动斑块上。
Phys Rev E. 2018 Jul;98(1-1):012125. doi: 10.1103/PhysRevE.98.012125.
8
Morphology of fine-particle monolayers deposited on nanopatterned substrates.沉积在纳米图案化衬底上的细颗粒单层的形态学。
Phys Rev E Stat Nonlin Soft Matter Phys. 2008 Mar;77(3 Pt 1):031603. doi: 10.1103/PhysRevE.77.031603. Epub 2008 Mar 5.

引用本文的文献

1
Experimental study of a nanoscale translocation ratchet.纳米尺度 translocation 棘轮的实验研究。
Proc Natl Acad Sci U S A. 2022 Jul 26;119(30):e2202527119. doi: 10.1073/pnas.2202527119. Epub 2022 Jul 18.

本文引用的文献

3
"Burnt-bridge" mechanism of molecular motor motion.分子马达运动的“断桥”机制
Phys Rev E Stat Nonlin Soft Matter Phys. 2005 Oct;72(4 Pt 2):046104. doi: 10.1103/PhysRevE.72.046104. Epub 2005 Oct 6.
5
What drives the translocation of stiff chains?是什么驱动了刚性链的易位?
Proc Natl Acad Sci U S A. 2003 Jul 22;100(15):8649-53. doi: 10.1073/pnas.1533334100. Epub 2003 Jul 8.
8
Directed particle diffusion under "burnt bridges" conditions.“断桥”条件下的定向粒子扩散
Phys Rev E Stat Nonlin Soft Matter Phys. 2001 Jul;64(1 Pt 1):011102. doi: 10.1103/PhysRevE.64.011102. Epub 2001 Jun 11.
9
Voltage-driven DNA translocations through a nanopore.电压驱动的DNA通过纳米孔的转位。
Phys Rev Lett. 2001 Apr 9;86(15):3435-8. doi: 10.1103/PhysRevLett.86.3435.

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验