Ghiringhelli G, Piazzalunga A, Dallera C, Schmitt T, Strocov V N, Schlappa J, Patthey L, Wang X, Berger H, Grioni M
CNR-INFM Coherentia and Soft, Dipartimento di Fisica, Politecnico di Milano, piazza Leonardo da Vinci 32, I-20133 Milano, Italy.
Phys Rev Lett. 2009 Jan 16;102(2):027401. doi: 10.1103/PhysRevLett.102.027401. Epub 2009 Jan 12.
We present high resolution (DeltaE=120 meV) resonant inelastic x-ray scattering data measured at the Ni L3 edge (2p_{3/2}-->3d) on the paradigmatic antiferromagnetic oxide NiO. Spectra reveal clear signatures of magnetic excitations at approximately 95 and approximately 190 meV whose energy seems independent from transferred momentum. These spectral features are well reproduced by a single Ni2+ ion model in an effective exchange field. Within this local model the two magnetic excitations are characterized by a variation of the atomic magnetic moment along the local ordering direction (DeltaS_{alpha}) of one and two units. The DeltaS_{alpha}=2 case has different nature from bimagnons observed in optical Raman spectra, for which DeltaS_{alpha}=0.
我们展示了在典型反铁磁氧化物NiO的Ni L3边缘(2p_{3/2}→3d)处测量的高分辨率(ΔE = 120 meV)共振非弹性X射线散射数据。光谱揭示了在约95 meV和约190 meV处磁激发的清晰特征,其能量似乎与转移动量无关。这些光谱特征通过有效交换场中的单个Ni2+离子模型得到了很好的再现。在这个局部模型中,两个磁激发的特征是原子磁矩沿局部有序方向(ΔS_{α})变化一个和两个单位。ΔS_{α}= 2的情况与光学拉曼光谱中观察到的双磁子性质不同,后者的ΔS_{α}= 0。