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[采用二氧化碳、氧气和四氟化碳液体气溶胶喷雾靶的激光产生等离子体源的光谱]

[The spectra of a laser-produced plasma source with CO2, O2 and CF4 liquid aerosol spray target].

作者信息

Ni Qi-Liang, Chen Bo

机构信息

State Key Lab of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China.

出版信息

Guang Pu Xue Yu Guang Pu Fen Xi. 2008 Nov;28(11):2465-8.

Abstract

A laser-produced plasma (LPP) source with liquid aerosol spray target and nanosecond laser was developed, based on both soft X-ray radiation metrology and extreme ultraviolet projection lithography (EUVL). The LPP source is composed of a stainless steel solenoid valve whose temperature can be continuously controlled, a Nd : YAG laser with pulse width, working wavelength and pulse energy being 7 ns, 1.064 microm and 1J respectively, and a pulse generator which can synchronously control the valve and the laser. A standard General Valve Corporation series 99 stainless steel solenoid valve with copper gasket seals and a Kel-F poppet are used in order to minimize leakage and poppet deformation during high-pressure cryogenic operation. A close fitting copper cooling jacket surrounds the valve body. The jacket clamps a copper coolant carrying tube 3 mm in diameter, which is fed by an automatically pressurized liquid nitrogen-filled dewar. The valve temperature can be controlled between 77 and 473 K. For sufficiently high backing pressure and low temperature, the valve reservoir gas can undergo a gas-to-liquid phase transition. Upon valve pulsing, the liquid is ejected into a vacuum and breaks up into droplets, which is called liquid aerosol spray target. For the above-mentioned LPP source, firstly, by the use of Cowan program on the basis of non-relativistic quantum mechanics, the authors computed the radiative transition wavelengths and probabilities in soft X-ray region for O4+, O5+, O6+, O7+, F5+, F6+ and F7+ ions which were correspondingly produced from the interaction of the 10(11)-10(12) W x cm(-2) power laser with liquid O2, CO2 and CF4 aerosol spray targets. Secondly, the authors measured the spectra of liquid O2, CO2 and CF4 aerosol spray target LPP sources in the 6-20 nm band for the 8 x 10(11) W x cm(-2) laser irradiance. The measured results were compared with the Cowan calculated results ones, and the radiative transition wavelength and probability for the measured spectral lines were obtained.

摘要

基于软X射线辐射计量学和极紫外投影光刻技术(EUVL),开发了一种带有液体气溶胶喷雾靶和纳秒激光的激光产生等离子体(LPP)源。该LPP源由一个温度可连续控制的不锈钢电磁阀、一个脉冲宽度为7 ns、工作波长为1.064微米、脉冲能量为1J的Nd:YAG激光器以及一个可同步控制阀门和激光器的脉冲发生器组成。为了使高压低温运行期间的泄漏和提升阀变形最小化,使用了标准的通用阀门公司99系列不锈钢电磁阀,其带有铜垫圈密封和凯尔氟提升阀。一个紧密配合的铜冷却套环绕着阀体。该冷却套夹住一根直径为3毫米的铜冷却剂输送管,该输送管由一个自动加压的液氮杜瓦瓶供给。阀门温度可控制在77至473 K之间。对于足够高的背压和低温,阀门储存器中的气体可发生气-液相转变。阀门脉冲触发时,液体被喷射到真空中并破碎成液滴,这被称为液体气溶胶喷雾靶。对于上述LPP源,首先,作者基于非相对论量子力学使用考恩程序,计算了10(11)-10(12) W x cm(-2)功率的激光与液体O2、CO2和CF4气溶胶喷雾靶相互作用时相应产生的O4+、O5+、O6+、O7+、F5+、F6+和F7+离子在软X射线区域的辐射跃迁波长和概率。其次,作者测量了8 x 10(11) W x cm(-2)激光辐照下液体O2、CO2和CF4气溶胶喷雾靶LPP源在6 - 20 nm波段的光谱。将测量结果与考恩计算结果进行比较,得到了测量谱线的辐射跃迁波长和概率。

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