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中国北京两年采样期内人为源与地质源对大气总悬浮颗粒物的贡献及其变化

Anthropogenic versus geogenic contribution to total suspended atmospheric particulate matter and its variations during a two-year sampling period in Beijing, China.

作者信息

Schleicher Nina, Norra Stefan, Chai Fahe, Chen Yizhen, Wang Shulan, Stüben Doris

机构信息

Institute of Mineralogy and Geochemistry, Universität Karlsruhe (TH), Adenauerring 20, 76131, Karlsruhe, Germany.

出版信息

J Environ Monit. 2010 Feb;12(2):434-41. doi: 10.1039/b914739j. Epub 2009 Nov 16.

Abstract

Weekly samples of total suspended particles in air (TSP) were taken in south-east Beijing for a two-year period continuously from August 2005 to August 2007. Mass concentrations varied between 76 and 1028 microg m(-3) with an average concentration of 370 microg m(-3) for the whole period. The chemical composition and the mass concentration of aerosols in combination with meteorological data are reflecting specific influences of distinct aerosol sources on the pollution of Beijing's atmosphere. Lead (Pb), titanium (Ti), zinc (Zn) and copper (Cu) concentrations were chosen as indicator elements for different sources. Their amounts considerably varied over the course of the year. Element ratios, such as Pb/Ti, supported the distinction between periods of predominant geogenic or anthropogenic caused pollution. However, the interactions between aerosols from different sources are numerous and aerosol pollution still is a big and complex challenge for the sustainable development of Beijing.

摘要

2005年8月至2007年8月期间,在北京东南部连续两年每周采集空气中总悬浮颗粒物(TSP)样本。整个期间,质量浓度在76至1028微克/立方米之间变化,平均浓度为370微克/立方米。气溶胶的化学成分和质量浓度与气象数据相结合,反映了不同气溶胶源对北京大气污染的特定影响。选择铅(Pb)、钛(Ti)、锌(Zn)和铜(Cu)的浓度作为不同来源的指示元素。它们的含量在一年中变化很大。元素比率,如Pb/Ti,有助于区分主要由地质成因或人为造成污染的时期。然而,不同来源气溶胶之间的相互作用众多,气溶胶污染仍然是北京可持续发展面临的一个重大而复杂的挑战。

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