Suppr超能文献

石墨烯量子点的分数填充简并壳中的磁性和相关性。

Magnetism and correlations in fractionally filled degenerate shells of graphene quantum dots.

机构信息

Institute for Microstructural Sciences, National Research Council of Canada, Ottawa, Canada.

出版信息

Phys Rev Lett. 2009 Dec 11;103(24):246805. doi: 10.1103/PhysRevLett.103.246805. Epub 2009 Dec 10.

Abstract

We show that the ground state and magnetization of the macroscopically degenerate shell of electronic states in triangular gated graphene quantum dots depends on the filling fraction of the shell. The effect of degeneracy, finite size, and electron-electron interactions are treated nonperturbatively using a combination of density functional theory, tight-binding, Hartree-Fock and configuration interaction methods. We show that electronic correlations play a crucial role in determining the nature of the ground state as a function of filling fraction of the degenerate shell at the Fermi level. We find that the half-filled charge neutral shell leads to full spin polarization but this magnetic moment can be completely destroyed by adding a single electron.

摘要

我们表明,在三角栅控石墨烯量子点中,电子态宏观简并壳层的基态和磁化强度取决于壳层的填充分数。使用密度泛函理论、紧束缚、哈特ree-Fock 和组态相互作用方法的组合,我们非微扰地处理了简并、有限大小和电子-电子相互作用的影响。我们表明,电子相关在确定基态的性质方面起着至关重要的作用,这是作为费米能级处简并壳层填充分数的函数。我们发现,半满的中性电荷壳层导致完全的自旋极化,但通过添加单个电子可以完全破坏这个磁矩。

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验