Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550, USA.
Phys Rev Lett. 2010 Feb 12;104(6):064801. doi: 10.1103/PhysRevLett.104.064801.
Intense and ultrashort x-ray pulses from free-electron lasers open up the possibility for near-atomic resolution imaging without the need for crystallization. Such experiments require high photon fluences and pulses shorter than the time to destroy the sample. We describe results with a new femtosecond pump-probe diffraction technique employing coherent 0.1 keV x rays from the FLASH soft x-ray free-electron laser. We show that the lifetime of a nanostructured sample can be extended to several picoseconds by a tamper layer to dampen and quench the sample explosion, making <1 nm resolution imaging feasible.
自由电子激光产生的高强度超短 X 射线脉冲为无需结晶即可实现近原子分辨率成像开辟了可能性。此类实验需要高光子通量和短于破坏样品所需时间的脉冲。我们利用 FLASH 软 X 射线自由电子激光产生的相干 0.1 keV X 射线,介绍了一种新的皮秒泵浦探测衍射技术的实验结果。我们证明,通过钝体层来阻尼和熄灭样品爆炸,可以将纳米结构样品的寿命延长至数皮秒,从而实现<1nm 分辨率成像。