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等离子体相互作用的单个CdSe/ZnS量子点的反聚束和发光闪烁抑制

Anti-bunching and luminescence blinking suppression from plasmon-interacted single CdSe/ZnS quantum dot.

作者信息

Wu Xiao-Wei, Gong Ming, Dong Chun-Hua, Cui Jin-Ming, Yang Yong, Sun Fang-Wen, Guo Guang-Can, Han Zheng-Fu

机构信息

Key Laboratory of Quantum Information, CAS, University of Science and Technology of China, Hefei 230026, China.

出版信息

Opt Express. 2010 Mar 15;18(6):6340-6. doi: 10.1364/OE.18.006340.

Abstract

CdSe/ZnS colloidal quantum dots generally exist as blinking phenomena during the luminescence process that remarkably influences its applications. In this work, we used the surface plasmonic effect to effectively modulate single quantum dots. Obvious contrasts have been observed by comparing single quantum dots on silica and gold films. The surface plasmon is shown to obviously suppress the blinking of single quantum dots. With further demonstrated second- order correlation measurements, an anti-bunching effect was observed. The anti-bunching dip gives the smallest value of g(2)(0) = 0.15, and the lifetime of the exciton has been reduced. This method presents the application's potential towards tunable high-emitting-speed single photon sources at room temperature.

摘要

CdSe/ZnS 胶体量子点在发光过程中通常会出现闪烁现象,这对其应用产生了显著影响。在这项工作中,我们利用表面等离子体效应有效地调制单个量子点。通过比较二氧化硅和金膜上的单个量子点,观察到了明显的差异。结果表明,表面等离子体能够显著抑制单个量子点的闪烁。通过进一步的二阶关联测量,观察到了反聚束效应。反聚束凹陷给出了最小的 g(2)(0) 值为 0.15,并且激子的寿命缩短了。该方法展示了在室温下实现可调谐高发射速度单光子源的应用潜力。

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