Institut für Theoretische Physik, Universität Leipzig, Postfach 100920, 04009 Leipzig, Germany.
Phys Rev Lett. 2010 Aug 27;105(9):090604. doi: 10.1103/PhysRevLett.105.090604. Epub 2010 Aug 26.
We derive the markovian description for the nonequilibrium brownian motion of a heated nanoparticle in a simple solvent with a temperature-dependent viscosity. Our analytical results for the generalized fluctuation-dissipation and Stokes-Einstein relations compare favorably with measurements of laser-heated gold nanoparticles and provide a practical rational basis for emerging photothermal tracer and nanoparticle trapping and tracking techniques.
我们推导出了在具有依赖温度的粘性的简单溶剂中加热的纳米粒子的非平衡布朗运动的马尔可夫描述。我们对广义涨落耗散和斯托克斯-爱因斯坦关系的分析结果与激光加热的金纳米粒子的测量结果进行了很好的比较,并为新兴的光热示踪和纳米粒子捕获和跟踪技术提供了实用的合理基础。