Department of Physics, University of Missouri-Kansas City, Kansas City, MO 64110, USA.
J Phys Condens Matter. 2010 Nov 10;22(44):443201. doi: 10.1088/0953-8984/22/44/443201. Epub 2010 Oct 22.
Detection of neutrons, at high total efficiency, with greater resolution in kinetic energy, time and/or real-space position, is fundamental to the advance of subfields within nuclear medicine, high-energy physics, non-proliferation of special nuclear materials, astrophysics, structural biology and chemistry, magnetism and nuclear energy. Clever indirect-conversion geometries, interaction/transport calculations and modern processing methods for silicon and gallium arsenide allow for the realization of moderate- to high-efficiency neutron detectors as a result of low defect concentrations, tuned reaction product ranges, enhanced effective omnidirectional cross sections and reduced electron-hole pair recombination from more physically abrupt and electronically engineered interfaces. Conversely, semiconductors with high neutron cross sections and unique transduction mechanisms capable of achieving very high total efficiency are gaining greater recognition despite the relative immaturity of their growth, lithographic processing and electronic structure understanding. This review focuses on advances and challenges in charged-particle-based device geometries, materials and associated mechanisms for direct and indirect transduction of thermal to fast neutrons within the context of application. Calorimetry- and radioluminescence-based intermediate processes in the solid state are not included.
高总探测效率、高能量分辨率、高时间分辨率和/或高位置分辨率的中子探测技术是核医学、高能物理、特殊核材料不扩散、天体物理、结构生物学和化学、磁学和核能等领域发展的基础。巧妙的间接转换几何结构、相互作用/输运计算和硅及砷化镓的现代加工方法使得具有中等至高探测效率的中子探测器成为可能,这是因为低缺陷浓度、调谐的反应产物射程、增强的有效各向同性横截面以及更物理性的陡化和更电子工程化的界面减少了电子-空穴对的复合。相反,尽管它们的生长、光刻加工和电子结构理解还相对不成熟,具有高中子截面和独特的转换机制、能够实现非常高总探测效率的半导体正获得越来越多的关注。本文综述了应用背景下基于带电粒子的器件几何结构、材料和相关热中子到快中子直接和间接转换机制的进展和挑战。不包括固态中的量热法和发光法等中间过程。