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准一维导体 K0.3MoO3 中的集体激发

Collective excitations in the quasi-one-dimensional conductor K0.3MoO3.

机构信息

Department of Physics, Faculty of Science, University of Split, Split, Croatia.

出版信息

J Phys Condens Matter. 2010 Dec 8;22(48):485603. doi: 10.1088/0953-8984/22/48/485603. Epub 2010 Nov 16.

Abstract

We investigate collective mode dispersions for the tight-binding dielectric matrix with two one-dimensional electron bands and the three-dimensional long-range Coulomb electron-electron interaction within the random phase approximation. The hybridized collective modes are the result of coupling between the intraband plasmon and the interband dipolar mode due to monopole-dipole Coulomb interaction. Our calculations show the existence of the renormalized plasmon mode below and the dipolar mode above the interband electron-hole quasi-continuum in the long-wavelength limit, as well as a distinct experimentally observable feature in the energy-loss function for large wavevectors in the region of interband excitations. The modes and features obtained are brought into correspondence with the data obtained from electron energy-loss spectroscopy measurements on a quasi-one-dimensional metal, the blue bronze K(0.3)MoO(3).

摘要

我们在随机相位近似下研究了具有两个一维电子能带和三维长程库仑电子-电子相互作用的紧束缚介电矩阵的集体模式色散。混合集体模式是由于单极-偶极库仑相互作用导致的带内等离子体和带间偶极模式之间耦合的结果。我们的计算表明,在长波极限下,在带间电子-空穴准连续体下方存在归一化等离子体模式,在带间激发区域的大波矢处的能量损失函数中存在明显的实验可观测特征。获得的模式和特征与从准一维金属蓝青铜 K(0.3)MoO(3)的电子能量损失谱测量中获得的数据相对应。

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