Leung Gong Wai, Vickers Mary E, Fix Thomas, Blamire Mark G
Department of Materials Science and Metallurgy, University of Cambridge, Pembroke Street, Cambridge CB2 3QZ, UK.
J Phys Condens Matter. 2009 Oct 21;21(42):426003. doi: 10.1088/0953-8984/21/42/426003. Epub 2009 Sep 29.
We report that the La(0.35)Sr(0.65)Ti(1-x)Fe(x)O(3) system forms a solid solution within the composition range 0≤x≤0.5 and a room temperature magnetic semiconductor phase exists at x = 0.20. This system shows an anomalous Hall effect and is ferromagnetic with a large moment per Fe ion. The results show that the strong La doping provides sufficient carriers to the system to maintain carrier-mediated ferromagnetism for low Fe doping. Furthermore, the presence of ferromagnetism within this phase space raises the possibility that the conduction, and hence the magnetism, could be electronically controlled.
我们报道了La(0.35)Sr(0.65)Ti(1 - x)Fe(x)O(3)体系在0≤x≤0.5的组成范围内形成固溶体,且在x = 0.20时存在室温磁性半导体相。该体系表现出反常霍尔效应,并且是具有每个铁离子较大磁矩的铁磁体。结果表明,强镧掺杂为该体系提供了足够的载流子,以在低铁掺杂情况下维持载流子介导的铁磁性。此外,在该相空间内铁磁性的存在增加了传导以及因此磁性可以通过电子方式控制的可能性。