Department of NanoBiophotonics, Max Planck Institute for Biophysical Chemistry, Göttingen, Germany.
Phys Rev Lett. 2011 Jul 1;107(1):017601. doi: 10.1103/PhysRevLett.107.017601.
We show stimulated emission depletion microscopy to break the diffraction limit in the all-far-field-optical detection of magnetic fields and resonances. Electron spin resonances from single nitrogen-vacancy centers in diamond located at subdiffraction proximities are fully discerned. Since diffraction is overcome by disallowing the signaling state through an optical transition such as stimulated emission, the spin state remains unaffected and amenable to microwave manipulation. Stimulated emission depletion presents a universal scheme for superresolving spin resonances detectable by fluorescence.
我们展示了受激发射损耗显微镜,以突破全远场光学检测磁场和共振的衍射极限。位于亚衍射近邻处的钻石中单个氮空位中心的电子自旋共振被完全分辨出来。由于通过诸如受激发射这样的光学跃迁来禁止信号状态,从而克服了衍射,因此自旋状态保持不变并且可进行微波操作。受激发射损耗为通过荧光可检测的自旋共振的超分辨提供了一种通用方案。