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在重力作用下,活性胶体悬浮液表现出极性有序性。

Active colloidal suspensions exhibit polar order under gravity.

机构信息

Institut für Theoretische Physik, Technische Universität Berlin, Hardenbergstrasse 36, 10623 Berlin, Germany.

出版信息

Phys Rev Lett. 2011 Jul 29;107(5):058301. doi: 10.1103/PhysRevLett.107.058301. Epub 2011 Jul 28.

Abstract

Recently, the steady sedimentation profile of a dilute suspension of chemically powered colloids was studied experimentally [J. Palacci et al., Phys. Rev. Lett. 105, 088304 (2010)]. It was found that the sedimentation length increases quadratically with the swimming speed of the active Brownian particles. Here we investigate theoretically the sedimentation of self-propelled particles undergoing translational and rotational diffusion. We find that the measured increase of the sedimentation length is coupled to a partial alignment of the suspension with the mean swimming direction oriented against the gravitational field. We suggest realistic parameter values to observe this polar order. Furthermore, we find that the dynamics of the active suspension can be derived from a generalized free energy functional.

摘要

最近,人们通过实验研究了化学动力胶体稀悬浮液的稳定沉降剖面[J. Palacci 等人,Phys. Rev. Lett. 105, 088304 (2010)]。结果发现,沉降长度与活性布朗粒子的游动速度呈二次方关系增加。在这里,我们从理论上研究了经历平移和旋转扩散的自推进粒子的沉降。我们发现,所测量的沉降长度的增加与悬浮液的部分对准有关,即悬浮液的平均游动方向与重力场相反。我们提出了观察这种极向有序的实际参数值。此外,我们发现活性悬浮液的动力学可以从广义自由能泛函中推导出来。

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