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交流:金属玻璃与其他玻璃有何不同?高频动力学的深入观察。

Communication: are metallic glasses different from other glasses? A closer look at their high frequency dynamics.

机构信息

Dpt. de Fisica Aplicada, UPC, E-08860 Castelldefels, Spain.

出版信息

J Chem Phys. 2011 Sep 14;135(10):101101. doi: 10.1063/1.3640002.

Abstract

Using high resolution inelastic x-ray scattering we studied the collective dynamics of the Pd(77)Si(16.5)Cu(6.5) metallic glass, focusing on the energy-momentum region where the boson peak appears. The dispersion relation and the width of the acoustic excitations are determined showing how the longitudinal acoustic modes maintain their dispersive character for frequencies well above the boson peak frequencies. Moreover, we prove that close to these frequencies there is a softening of the apparent sound speed indicating a failure of the Debye continuum approximation at the boson peak frequencies and challenging previous results on other metallic glasses.

摘要

我们使用高分辨率非弹性 X 射线散射研究了 Pd(77)Si(16.5)Cu(6.5)金属玻璃的集体动力学,重点关注出现玻色峰的能量-动量区域。我们确定了色散关系和声学激发的宽度,表明纵向声学模式如何在远高于玻色峰频率的频率下保持其色散特性。此外,我们证明在这些频率附近,表观声速会软化,表明在玻色峰频率处德拜连续体近似失效,并对其他金属玻璃的先前结果提出了挑战。

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