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钕镍酸锶中绝缘-金属相变附近的莫特物理学。

Mott physics near the insulator-to-metal transition in NdNiO3.

机构信息

Department of Physics, University of California-San Diego, La Jolla, California 92093, USA.

出版信息

Phys Rev Lett. 2011 Oct 21;107(17):176401. doi: 10.1103/PhysRevLett.107.176401. Epub 2011 Oct 17.

DOI:10.1103/PhysRevLett.107.176401
PMID:22107544
Abstract

An optical study of NdNiO(3) ultrathin films with insulating and metallic ground states reveals new aspects of the insulator-to-metal transition that point to Mott physics as the driving force. In contrast with the behavior of charge-ordered systems, we find that the emergence of the Drude resonance across the transition is linked to a spectral weight transfer over an energy range of the order of the Coulomb repulsion U, as the energy gap is filled with states instead of closing continuously.

摘要

对具有绝缘和金属基态的 NdNiO(3) 超薄薄膜进行的光学研究揭示了绝缘-金属转变的新方面,表明莫特物理是驱动力。与电荷有序系统的行为相反,我们发现,在转变过程中 Drude 共振的出现与在库仑排斥 U 量级的能量范围内的光谱权重转移有关,因为能隙被填充而不是连续关闭。

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