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中国太湖水中多环芳烃的生态风险特征。

Characterizing ecological risk for polycyclic aromatic hydrocarbons in water from Lake Taihu, China.

机构信息

Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China.

出版信息

Environ Monit Assess. 2012 Nov;184(11):6815-25. doi: 10.1007/s10661-011-2460-5. Epub 2011 Nov 29.

Abstract

Lake Taihu provides vital ecological services for humans in China; it receives a great deal of attention regarding its ecological and environmental conditions. In this study, the ecological risks of eight individual polycyclic aromatic hydrocarbons (PAHs) in water were assessed using probabilistic distributions of the hazard quotient based on Monte Carlo simulation. The results show that the 95th percentile of the hazard quotients ranged from 0.00074 to 2.831, and the ecological risk of Flua was highest, followed by, in descending order of risk, B[a]P > Pyr > Ant > Phe > Flu > Ace > Chr. The probabilities of hazard quotients exceeding a decision criteria of 0.3 were 18.09%, 6.51%, 3.76%, and 2.85% for Flua, B[a]P, Pyr, and Ant, respectively, indicating their potential ecological risks to aquatic organisms. The spatial distribution of hazard quotients for these four individual PAHs with potential ecological risk were obtained using Geographic Information System (GIS), and similar spatial distribution patterns were also observed in the lake. The highest ecological risks of these four individual PAHs to aquatic organisms were found in Meiliang Bay, followed by Gonghu Bay and Xukou Bay. The uncertainty within the ecological risk assessment was also discussed.

摘要

太湖为中国的人类提供了重要的生态服务;它的生态和环境条件受到了广泛关注。在本研究中,采用基于蒙特卡罗模拟的危害商概率分布来评估八种单体多环芳烃(PAHs)在水中的生态风险。结果表明,危害商的第 95 百分位数范围为 0.00074 至 2.831,苊的生态风险最高,其次是苯并[a]芘、苊烯、蒽、菲、荧蒽、芘、屈。危害商超过 0.3 决策标准的概率分别为苊的 18.09%、苯并[a]芘的 6.51%、苊烯的 3.76%和蒽的 2.85%,表明它们对水生生物具有潜在的生态风险。利用地理信息系统(GIS)获得了这四种具有潜在生态风险的单体 PAHs 的危害商空间分布,在湖中也观察到了相似的空间分布模式。这四种单体 PAHs 对水生生物的最高生态风险出现在梅梁湾,其次是贡湖湾和胥口湾。还讨论了生态风险评估中的不确定性。

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