Department of Chemistry and the Materials Research Center, Northwestern University, 2145 Sheridan Road, Evanston, Illinois 60208, USA.
ACS Appl Mater Interfaces. 2012 Mar;4(3):1614-9. doi: 10.1021/am201776p. Epub 2012 Feb 24.
Solution processing of amorphous metal oxide materials to fabricate thin-film transistors (TFTs) has received great recent interest. We demonstrate here an optimized "ink" and printing process for inkjet patterning of amorphous indium gallium zinc oxide (a-IGZO) TFTs and investigate the effects of device structure on derived electron mobility. Bottom-gate top-contact (BGTC) TFTs are fabricated and shown to exhibit electron mobilities comparable to a-Si:H. Furthermore, a record electron mobility of 2.5 cm(2) V(-1) s(-1) is demonstrated for bottom-gate bottom-contact (BGBC) TFTs. The mechanism underlying such impressive performance is investigated using transmission line techniques, and it is shown that the semiconductor-source/drain electrode interface contact resistance is nearly an order of magnitude lower for BGBC transistors versus BGTC devices.
非晶态金属氧化物材料的溶液处理在制造薄膜晶体管(TFT)方面引起了极大的关注。我们在此展示了一种优化的“墨水”和喷墨打印工艺,用于喷墨打印非晶态铟镓锌氧化物(a-IGZO)TFT,并研究了器件结构对衍生电子迁移率的影响。制备了底栅顶接触(BGTC)TFT,并证明其电子迁移率可与非晶硅(a-Si:H)相媲美。此外,还展示了底栅底接触(BGBC)TFT 的电子迁移率达到了 2.5 cm²/V·s 的记录值。使用传输线技术研究了这种出色性能的机理,结果表明,与 BGTC 器件相比,BGBC 晶体管的半导体源/漏电极界面接触电阻低了近一个数量级。