Department of Chemistry and Chemical Biology, Harvard University, Cambridge, Massachusetts 02138, USA.
J Am Chem Soc. 2012 Mar 7;134(9):4007-10. doi: 10.1021/ja211602t. Epub 2012 Feb 24.
Integration of catalytic nanostructured platinum and palladium within 3D microscale structures or fluidic environments is important for systems ranging from micropumps to microfluidic chemical reactors and energy converters. We report a straightforward procedure to fabricate microscale patterns of nanocrystalline platinum and palladium using multiphoton lithography. These materials display excellent catalytic, electrical, and electrochemical properties, and we demonstrate high-resolution integration of catalysts within 3D defined microenvironments to generate directed autonomous particle and fluid transport.
在 3D 微尺度结构或流体环境中集成催化纳米结构的铂和钯对于从微泵到微流控化学反应器和能量转换器的系统非常重要。我们报告了一种使用多光子光刻技术制造纳米晶铂和钯微尺度图案的简单方法。这些材料表现出优异的催化、电学和电化学性能,并且我们展示了在 3D 定义的微环境中高分辨率集成催化剂,以产生定向自主粒子和流体输送。