Wang Xu-Jie, Huang Guoqi, Li Ming-Yang, Wang Yuan-Zhuo, Liu Li, Wu Bang, Liu Hanqing, Ni Haiqiao, Niu Zhichuan, Ji Weijie, Jiao Rongzhen, Yin Hua-Lei, Yuan Zhiliang
Beijing Academy of Quantum Information Sciences, Beijing, China.
School of Science, Beijing University of Posts and Telecommunications, Beijing, China.
Nat Commun. 2025 Jul 12;16(1):6453. doi: 10.1038/s41467-025-61884-x.
Resonance fluorescence of a two-level emitter displays persistently anti-bunching irrespective of the excitation intensity, but inherits the driving laser's linewidth under weak monochromatic excitation. These properties are commonly explained in terms of two disjoined pictures, i.e., the emitter's single photon saturation or passively scattering light. Here, we propose a unified model that treats all fluorescence photons as spontaneous emission, one at a time, and can explain simultaneously both the spectral and correlation properties of the emission. We theoretically derive the excitation power dependencies, measurable at the single-photon incidence level, of the first-order coherence of the whole resonance fluorescence and super-bunching of the spectrally filtered, followed by experimental confirmation on a semiconductor quantum dot micro-pillar device. Furthermore, our model explains peculiar coincidence bunching observed in phase-dependent two-photon interference experiments. Our work provides an intuitive understanding of coherent light-matter interaction and may stimulate new applications.
两能级发射体的共振荧光无论激发强度如何都持续呈现反聚束现象,但在弱单色激发下会继承驱动激光的线宽。这些特性通常用两个不相关的图像来解释,即发射体的单光子饱和或被动散射光。在这里,我们提出了一个统一模型,该模型将所有荧光光子都视为一次一个的自发发射,并且可以同时解释发射的光谱和相关特性。我们从理论上推导出在单光子入射水平可测量的全共振荧光的一阶相干性和光谱滤波后的超聚束的激发功率依赖性,随后在半导体量子点微柱器件上进行了实验验证。此外,我们的模型解释了在相位相关的双光子干涉实验中观察到的特殊符合聚束现象。我们的工作为相干光与物质相互作用提供了直观理解,并可能激发新的应用。