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台湾食品中的多溴联苯醚:水平及人体膳食暴露评估。

Polybrominated diphenyl ethers in foodstuffs from Taiwan: level and human dietary exposure assessment.

机构信息

Institute of Environmental and Occupational Health Sciences, College of Medicine, National Yang-Ming University, Shi-Pai, Taipei, Taiwan.

出版信息

Sci Total Environ. 2012 Aug 1;431:183-7. doi: 10.1016/j.scitotenv.2012.05.046. Epub 2012 Jun 7.

Abstract

Polybrominated diphenyl ethers (PBDEs) may contaminate food through bioconcentration and biomagnification. PBDEs often exist in the food chain and are consumed by humans. This study aims to determine the concentrations of PBDEs in food intake and to estimate the daily exposure of Taiwanese citizens to PBDEs. One hundred and eight food samples from nine types of commonly consumed foodstuffs were collected from northern, central, southern, and eastern regions of Taiwan. The samples were analyzed for PBDE level by gas chromatography mass spectrometry. Also, a daily dietary intake survey was conducted of 466 adults (153 men, 313 women) in these four regions of Taiwan. Taiwanese daily dietary intake of PBDE is calculated by means of food PBDEs level and daily dietary intake. The result of this study showed the highest concentration of ΣPBDE was found in butter (890.3±309.0 pg/g wet weight), followed by egg and pork (553.0±185.0 pg/g wet weight and 545.4±181.0 pg/g wet weight). Deca-BDE was found the highest concentration among eight kinds PBDEs. The average daily intake of PBDEs for the 466 subjects was 67.95±23.01 ng/day. There was a significant difference between the daily intake of ΣPBDE in different regions of Taiwan (p<0.05). The highest daily intake of ΣPBDE was in northern Taiwan, which is also the most urbanized area.

摘要

多溴二苯醚(PBDEs)可能通过生物浓缩和生物放大作用污染食物。PBDEs 经常存在于食物链中,并被人类摄入。本研究旨在确定食物摄入中 PBDEs 的浓度,并估计台湾居民每日接触 PBDEs 的情况。从台湾北部、中部、南部和东部地区采集了 9 种常见食品的 108 个食品样本。这些样本通过气相色谱-质谱法进行了 PBDE 水平分析。此外,还对台湾这四个地区的 466 名成年人(153 名男性,313 名女性)进行了每日饮食摄入调查。通过食物 PBDE 水平和每日饮食摄入量计算台湾人每日 PBDE 饮食摄入量。本研究结果显示,ΣPBDE 的最高浓度出现在黄油中(890.3±309.0 pg/g 湿重),其次是鸡蛋和猪肉(553.0±185.0 pg/g 湿重和 545.4±181.0 pg/g 湿重)。在 8 种 PBDE 中,十溴二苯醚的浓度最高。466 名受试者的 PBDE 日均摄入量为 67.95±23.01 ng/天。台湾不同地区的 ΣPBDE 日摄入量存在显著差异(p<0.05)。北部地区的 ΣPBDE 日摄入量最高,该地区也是城市化程度最高的地区。

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