Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.
Proc Natl Acad Sci U S A. 2012 Nov 6;109(45):18332-7. doi: 10.1073/pnas.1209471109. Epub 2012 Oct 23.
A detailed phenomenology of low energy excitations is a crucial starting point for microscopic understanding of complex materials, such as the cuprate high-temperature superconductors. Because of its unique momentum-space discrimination, angle-resolved photoemission spectroscopy (ARPES) is ideally suited for this task in the cuprates, where emergent phases, particularly superconductivity and the pseudogap, have anisotropic gap structure in momentum space. We present a comprehensive doping- and temperature-dependence ARPES study of spectral gaps in Bi(2)Sr(2)CaCu(2)O(8+δ), covering much of the superconducting portion of the phase diagram. In the ground state, abrupt changes in near-nodal gap phenomenology give spectroscopic evidence for two potential quantum critical points, p = 0.19 for the pseudogap phase and p = 0.076 for another competing phase. Temperature dependence reveals that the pseudogap is not static below T(c) and exists p > 0.19 at higher temperatures. Our data imply a revised phase diagram that reconciles conflicting reports about the endpoint of the pseudogap in the literature, incorporates phase competition between the superconducting gap and pseudogap, and highlights distinct physics at the edge of the superconducting dome.
低能激发的详细现象学是理解复杂材料(如铜酸盐高温超导体)微观结构的关键起点。由于角分辨光电子能谱(ARPES)在铜酸盐中具有独特的动量空间分辨能力,非常适合于研究其中出现的各向异性能隙结构的相,特别是超导相和赝能隙。我们对 Bi(2)Sr(2)CaCu(2)O(8+δ)中的能带隙进行了全面的掺杂和温度依赖的 ARPES 研究,涵盖了相图中超导部分的大部分区域。在基态下,近节点能隙现象的突然变化为两个潜在量子临界点提供了光谱证据,一个临界点对应赝能隙相,临界点掺杂比 p = 0.19,另一个临界点对应另一个竞争相,临界点掺杂比 p = 0.076。温度依赖关系表明,在 T(c)以下,赝能隙不是静态的,在较高温度下存在 p > 0.19 的赝能隙。我们的数据表明了一个修订后的相图,该相图调和了文献中关于赝能隙终点的相互矛盾的报告,包含了超导能隙和赝能隙之间的竞争,以及在超导穹顶边缘的独特物理现象。