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双层栅 ABC 和 ABA 三嗪石墨烯的输运研究:非常大的垂直电场中的带隙打开和能带结构调谐。

Transport studies of dual-gated ABC and ABA trilayer graphene: band gap opening and band structure tuning in very large perpendicular electric fields.

机构信息

Department of Physics, The Pennsylvania State University, University Park, Pennsylvania 16802, USA.

出版信息

Nano Lett. 2013 Feb 13;13(2):369-73. doi: 10.1021/nl303375a. Epub 2013 Jan 30.

DOI:10.1021/nl303375a
PMID:23336322
Abstract

We report on the transport properties of ABC and ABA stacked trilayer graphene using dual, locally gated field effect devices. The high efficiency and large breakdown voltage of the HfO(2) top and bottom gates enable independent tuning of the perpendicular electric field and the Fermi level over an unprecedentedly large range. We observe a resistance change of 6 orders of magnitude in the ABC trilayer, which demonstrates the opening of a band gap. Our data suggest that the gap saturates at a large displacement field of D ~ 3 V/nm, in agreement with self-consistent Hartree calculations. In contrast, the ABA trilayer remains metallic even under a large perpendicular electric field. Despite the absence of a band gap, the band structure of the ABA trilayer continues to evolve with increasing D. We observe signatures of two-band conduction at large D fields. Our self-consistent Hartree calculation reproduces many aspects of the experimental data but also points to the need for more sophisticated theory.

摘要

我们报告了使用双局域门控场效应器件的 ABC 和 ABA 堆叠三层石墨烯的输运性质。HfO2顶栅和底栅的高效率和大击穿电压使得垂直电场和费米能级能够在前所未有的大范围内独立调节。我们在 ABC 三层石墨烯中观察到了 6 个数量级的电阻变化,这表明带隙的打开。我们的数据表明,间隙在大约 3 V/nm 的大位移场 D 处饱和,这与自洽的哈特ree 计算结果一致。相比之下,即使在大垂直电场下,ABA 三层石墨烯仍然保持金属性。尽管没有带隙,但 ABA 三层石墨烯的能带结构仍随着 D 的增加而继续演变。我们在大 D 场下观察到了双带传导的特征。我们的自洽哈特ree 计算再现了实验数据的许多方面,但也指出需要更复杂的理论。

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