Institut Néel, CNRS and Universite Joseph Fourier Grenoble, BP 166, 38042 Grenoble Cedex 9, France.
Phys Rev Lett. 2012 Dec 28;109(26):264301. doi: 10.1103/PhysRevLett.109.264301. Epub 2012 Dec 27.
Owing to its two-dimensional electronic structure, graphene exhibits many unique properties. One of them is a wave vector and temperature dependent plasmon in the infrared range. Theory predicts that due to these plasmons, graphene can be used as a universal material to enhance nanoscale radiative heat exchange for any dielectric substrate. Here we report on radiative heat transfer experiments between SiC and a SiO2 sphere that have nonmatching phonon polariton frequencies, and thus only weakly exchange heat in near field. We observed that the heat flux contribution of graphene epitaxially grown on SiC dominates at short distances. The influence of plasmons on radiative heat transfer is further supported with measurements for doped silicon. These results highlight graphene's strong potential in photonic near field and energy conversion devices.
由于其二维电子结构,石墨烯表现出许多独特的性质。其中之一是在红外范围内具有波矢和温度相关的等离子体。理论预测,由于这些等离子体,石墨烯可以用作通用材料,以增强任何介电衬底的纳米级辐射热交换。在这里,我们报告了在 SiC 和具有非匹配声子极化激元频率的 SiO2 球体之间的辐射热传递实验,因此在近场中仅弱地交换热量。我们观察到,在短距离内,生长在 SiC 上的石墨烯的热流贡献占主导地位。用掺杂硅进行的测量进一步支持了等离子体对辐射热传递的影响。这些结果突出了石墨烯在光子近场和能量转换器件中的强大潜力。