Molecular Imaging Center, National Taiwan University, Taipei 10617, Taiwan.
Nano Lett. 2013 Mar 13;13(3):1139-44. doi: 10.1021/nl3044986. Epub 2013 Feb 13.
The generation of guided acoustic phonons in the GHz range in GaN/AlN superlattices grown atop a GaN nanowire is presented. Combined with a femtosecond laser, ultrafast pump-probe spectroscopy allows the generation and detection of guided acoustic phonons at different frequencies in the nanowire superlattices. The capability of the nanowire superlattices to be excellent detectors of acoustic phonons at specific frequencies is then used to observe the strong dispersion, as a result of nanoconfinement, of guided acoustic phonons after their propagation in the nanowire. The generation of high frequency coherent guided acoustic phonons could be useful not only to realize an acoustic transducer with a nanolateral size but also as a source to understand the thermal behavior of nanowires.
本文提出了在 GaN 纳米线顶部生长的 GaN/AlN 超晶格中产生 GHz 范围的导声子的方法。结合飞秒激光,超快泵浦探测光谱学允许在纳米线超晶格中不同频率产生和检测导声子。然后,利用纳米线超晶格在特定频率下作为声子的优异探测器的能力,观察到导声子在纳米线中传播后的强色散,这是由于纳米限制的结果。高频相干导声子的产生不仅可用于实现具有纳米横向尺寸的声换能器,而且还可作为源来了解纳米线的热行为。