Schubert Martin, Grossmann Martin, He Chuan, Brick Delia, Scheel Patricia, Ristow Oliver, Gusev Vitalyi, Dekorsy Thomas
Department of Physics, University of Konstanz, Germany.
Department of Physics, University of Konstanz, Germany.
Ultrasonics. 2015 Feb;56:109-15. doi: 10.1016/j.ultras.2014.06.018. Epub 2014 Jul 24.
Single crystalline membranes are a perfect model system for the study of coherent acoustic phonon generation and decay in the time domain. Coherent acoustical modes are excited and detected in thin single-crystalline silicon and gallium arsenide membranes with femtosecond pulses in the ultraviolet and infrared wavelength region using the asynchronous optical sampling technique. The measured acoustic spectra are compared with each other and are discussed in terms of different generation and detection mechanisms. A clear dependence of the generated spectra on the absorption length of the pump and probe pulses is observed. It is shown that a short absorption length for the pump pulse leads to the generation of coherent high frequency phonons up to several 100 GHz frequencies. Membranes are demonstrated to be useful as broadband acoustic cavities and can help to disentangle details of high frequency phonon dynamics. Two-layer membrane systems offer additional insight into energy transfer in the GHz frequency range and adhesion properties.
单晶膜是用于研究时域中相干声子产生和衰减的理想模型系统。利用异步光学采样技术,在紫外和红外波长区域用飞秒脉冲激发并检测薄单晶硅和砷化镓膜中的相干声学模式。将测量的声谱相互比较,并根据不同的产生和检测机制进行讨论。观察到所产生的光谱对泵浦脉冲和探测脉冲的吸收长度有明显的依赖性。结果表明,泵浦脉冲的短吸收长度会导致产生高达数百吉赫兹频率的相干高频声子。膜被证明可用作宽带声学腔,并有助于厘清高频声子动力学的细节。双层膜系统能让人进一步了解吉赫兹频率范围内的能量转移和粘附特性。