Biophysics Program and the Department of Chemistry and Biochemistry, The Ohio State University, Columbus, Ohio 43210, USA.
J Biol Chem. 2013 Apr 19;288(16):11590-600. doi: 10.1074/jbc.M113.459982. Epub 2013 Mar 5.
Replicative DNA polymerases use a complex, multistep mechanism for efficient and accurate DNA replication as uncovered by intense kinetic and structural studies. Recently, single-molecule fluorescence spectroscopy has provided new insights into real time conformational dynamics utilized by DNA polymerases during substrate binding and nucleotide incorporation. We have used single-molecule Förster resonance energy transfer techniques to investigate the kinetics and conformational dynamics of Sulfolobus solfataricus DNA polymerase B1 (PolB1) during DNA and nucleotide binding. Our experiments demonstrate that this replicative polymerase can bind to DNA in at least three conformations, corresponding to an open and closed conformation of the finger domain as well as a conformation with the DNA substrate bound to the exonuclease active site of PolB1. Additionally, our results show that PolB1 can transition between these conformations without dissociating from a primer-template DNA substrate. Furthermore, we show that the closed conformation is promoted by a matched incoming dNTP but not by a mismatched dNTP and that mismatches at the primer-template terminus lead to an increase in the binding of the DNA to the exonuclease site. Our analysis has also revealed new details of the biphasic dissociation kinetics of the polymerase-DNA binary complex. Notably, comparison of the results obtained in this study with PolB1 with those from similar single-molecule studies with an A-family DNA polymerase suggests mechanistic differences between these polymerases. In summary, our findings provide novel mechanistic insights into protein conformational dynamics and substrate binding kinetics of a high fidelity B-family DNA polymerase.
复制 DNA 聚合酶利用复杂的多步骤机制实现高效和准确的 DNA 复制,这一机制在深入的动力学和结构研究中得到了揭示。最近,单分子荧光光谱学为 DNA 聚合酶在底物结合和核苷酸掺入过程中利用的实时构象动力学提供了新的见解。我们使用单分子荧光共振能量转移技术研究了 Sulfolobus solfataricus DNA 聚合酶 B1(PolB1)在 DNA 和核苷酸结合过程中的动力学和构象动力学。我们的实验表明,这种复制聚合酶可以以至少三种构象结合 DNA,对应于指状结构的开放和闭合构象,以及与 PolB1 的外切酶活性位点结合的 DNA 底物的构象。此外,我们的结果表明,PolB1 可以在不与引物-模板 DNA 底物解离的情况下在这些构象之间转换。此外,我们表明,封闭构象是由匹配的进入 dNTP 促进的,而不是由不匹配的 dNTP 促进的,并且引物-模板末端的不匹配会导致 DNA 与外切酶结合增加。我们的分析还揭示了聚合酶-DNA 二元复合物双相解离动力学的新细节。值得注意的是,将本研究中获得的 PolB1 与类似的 A 家族 DNA 聚合酶的单分子研究结果进行比较,表明这些聚合酶之间存在机制差异。总之,我们的研究结果为高保真 B 家族 DNA 聚合酶的蛋白质构象动力学和底物结合动力学提供了新的机制见解。