Wayne State University, Department of Pharmaceutical Sciences, 259 Mack Ave, Detroit, MI 48202, USA.
Bioorg Med Chem. 2013 Jun 1;21(11):3164-74. doi: 10.1016/j.bmc.2013.03.059. Epub 2013 Apr 1.
The goal of the present study was to explore, in our previously developed hybrid template, the effect of introduction of additional heterocyclic rings (mimicking catechol hydroxyl groups as bioisosteric replacement) on selectivity and affinity for the D3 versus D2 receptor. In addition, we wanted to explore the effect of derivatization of functional groups of the agonist binding moiety in compounds developed by us earlier from the hybrid template. Binding affinity (K(i)) of the new compounds was measured with tritiated spiperone as the radioligand and HEK-293 cells expressing either D2 or D3 receptors. Functional activity of selected compounds was assessed in the GTPγS binding assay. In the imidazole series, compound 10a exhibited the highest D3 affinity whereas the indole derivative 13 exhibited similar high D3 affinity. Functionalization of the amino group in agonist (+)-9d with different sulfonamides derivatives improved the D3 affinity significantly with (+)-14f exhibiting the highest affinity. However, functionalization of the hydroxyl and amino groups of 15 and (+)-9d, known agonist and partial agonist, to sulfonate ester and amide in general modulated the affinity. In both cases loss of agonist potency resulted from such derivatization.
本研究的目的是在我们之前开发的杂合模板中探索引入额外杂环(模拟儿茶酚羟基作为生物等排体取代)对 D3 与 D2 受体选择性和亲和力的影响。此外,我们还希望探索我们之前从杂合模板中开发的激动剂结合部分的官能团衍生化对化合物的影响。用氚标记的螺哌隆作为放射性配体,用表达 D2 或 D3 受体的 HEK-293 细胞测量新化合物的结合亲和力(K(i))。在 GTPγS 结合测定中评估选定化合物的功能活性。在咪唑系列中,化合物 10a 表现出最高的 D3 亲和力,而吲哚衍生物 13 表现出相似的高 D3 亲和力。用不同的磺酰胺衍生物对 (+)-9d 的氨基进行官能化,显著提高了 D3 亲和力,其中 (+)-14f 表现出最高的亲和力。然而,15 和 (+)-9d(已知的激动剂和部分激动剂)的羟基和氨基的官能化通常会调节亲和力。在这两种情况下,这种衍生化都会导致激动剂效力的丧失。