具有布朗斯台德和路易斯酸位点的沸石催化糠醛制备γ-戊内酯的多米诺反应 - Suppr

Domino reaction catalyzed by zeolites with Brønsted and Lewis acid sites for the production of γ-valerolactone from furfural.

作者信息

Bui Linh, Luo Helen, Gunther William R, Román-Leshkov Yuriy

机构信息

Department of Chemical Engineering, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, MA 02139, USA.

出版信息

Angew Chem Int Ed Engl. 2013 Jul 29;52(31):8022-5. doi: 10.1002/anie.201302575. Epub 2013 Jun 11.

DOI:10.1002/anie.201302575

PMID:23757377

Abstract

摘要

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Domino reaction catalyzed by zeolites with Brønsted and Lewis acid sites for the production of γ-valerolactone from furfural.具有布朗斯台德和路易斯酸位点的沸石催化糠醛制备γ-戊内酯的多米诺反应

Angew Chem Int Ed Engl. 2013 Jul 29;52(31):8022-5. doi: 10.1002/anie.201302575. Epub 2013 Jun 11.

A continuous flow strategy for the coupled transfer hydrogenation and etherification of 5-(hydroxymethyl)furfural using Lewis acid zeolites.一种使用路易斯酸沸石对5-(羟甲基)糠醛进行耦合转移氢化和醚化的连续流动策略。

ChemSusChem. 2014 Aug;7(8):2255-65. doi: 10.1002/cssc.201402100. Epub 2014 Jul 8.

Liquid-Phase Catalytic Transfer Hydrogenation of Furfural over Homogeneous Lewis Acid-Ru/C Catalysts.均相路易斯酸-钌/碳催化剂上糠醛的液相加氢。

ChemSusChem. 2015 Jun 22;8(12):2046-54. doi: 10.1002/cssc.201500212. Epub 2015 May 26.

Efficient solid acid catalyst containing Lewis and Brønsted Acid sites for the production of furfurals.用于糠醛生产的含有路易斯酸和布朗斯特酸位点的高效固体酸催化剂。

ChemSusChem. 2014 Aug;7(8):2342-50. doi: 10.1002/cssc.201402007. Epub 2014 May 7.

Efficient Conversion of Biomass-Derived Levulinic Acid to γ-Valerolactone over Polyoxometalate@Zr-Based Metal-Organic Frameworks: The Synergistic Effect of Bro̷nsted and Lewis Acidic Sites.多酸@Zr 基金属有机框架上生物质衍生的乙酰丙酸到γ-戊内酯的高效转化：Brønsted 和 Lewis 酸性位的协同作用。

Inorg Chem. 2021 Jun 7;60(11):7785-7793. doi: 10.1021/acs.inorgchem.1c00185. Epub 2021 Mar 23.

Synthesis of terephthalic acid via Diels-Alder reactions with ethylene and oxidized variants of 5-hydroxymethylfurfural.通过与乙烯的 Diels-Alder 反应以及 5-羟甲基糠醛的氧化变体合成对苯二甲酸。

Proc Natl Acad Sci U S A. 2014 Jun 10;111(23):8363-7. doi: 10.1073/pnas.1408345111. Epub 2014 May 27.

Lewis Acid Zeolites for Biomass Conversion: Perspectives and Challenges on Reactivity, Synthesis, and Stability.用于生物质转化的路易斯酸沸石：反应性、合成及稳定性方面的前景与挑战

Annu Rev Chem Biomol Eng. 2016 Jun 7;7:663-92. doi: 10.1146/annurev-chembioeng-080615-034551. Epub 2016 Apr 21.

Conversion of hemicellulose into furfural using solid acid catalysts in γ-valerolactone.在γ-戊内酯中使用固体酸催化剂将半纤维素转化为糠醛。

Angew Chem Int Ed Engl. 2013 Jan 21;52(4):1270-4. doi: 10.1002/anie.201207334. Epub 2012 Dec 4.

Orderly Layered Zr-Benzylphosphonate Nanohybrids for Efficient Acid-Base-Mediated Bifunctional/Cascade Catalysis.用于高效酸碱介导的双功能/级联催化的有序层状锆-苄基膦酸酯纳米杂化物

ChemSusChem. 2017 Feb 22;10(4):681-686. doi: 10.1002/cssc.201601570. Epub 2017 Jan 27.

Highly selective Lewis acid sites in desilicated MFI zeolites for dihydroxyacetone isomerization to lactic acid.脱硅 MFI 沸石中高选择性的路易斯酸位用于二羟丙酮异构化为乳酸。

ChemSusChem. 2013 May;6(5):831-9. doi: 10.1002/cssc.201200703. Epub 2013 Apr 3.

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High Selectivity and Yield in Catalytic Transfer Hydrogenation of Furfural to Furfuryl Alcohol by Zirconium Propoxide Modified Mesoporous Silica.丙醇锆改性介孔二氧化硅催化糠醛转移加氢制糠醇的高选择性和高收率

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Carbon Decorated Pd Species within Zeolite for Selective Furfural Hydrogenation.用于糠醛选择性加氢的沸石内碳修饰钯物种

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Catalytic Production and Upgrading of Furfural: A Platform Compound.糠醛的催化生产和升级：一种平台化合物。

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Spatial segregation of catalytic sites within Pd doped H-ZSM-5 for fatty acid hydrodeoxygenation to alkanes.钯掺杂的H-ZSM-5中用于脂肪酸加氢脱氧制烷烃的催化位点的空间分离。

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Zirconium Phosphate-Pillared Zeolite MCM-36 for Green Production of γ-Valerolactone from Levulinic Acid via Catalytic Transfer Hydrogenation.磷酸锆柱撑沸石MCM-36用于通过催化转移氢化从乙酰丙酸绿色生产γ-戊内酯

Molecules. 2024 Aug 9;29(16):3779. doi: 10.3390/molecules29163779.

Modulating acid sites in Y zeolite for valorisation of furfural to get γ-valerolactone.调节Y型沸石中的酸性位点以实现糠醛转化制备γ-戊内酯。

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Promoter Effect of Pt on Zr Catalysts to Increase the Conversion of Furfural to γ-Valerolactone Using Batch and Continuous Flow Reactors: Influence of the Way of the Incorporation of the Pt Sites.铂对锆催化剂的促进作用，通过间歇式和连续流动反应器提高糠醛向γ-戊内酯的转化率：铂位点引入方式的影响

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Critical Factors Affecting the Selective Transformation of 5-Hydroxymethylfurfural to 3-Hydroxymethylcyclopentanone Over Ni Catalysts.镍催化剂上影响5-羟甲基糠醛选择性转化为3-羟甲基环戊酮的关键因素

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Nb-Based Catalysts for the Valorization of Furfural into Valuable Product through in One-Pot Reaction.用于糠醛一锅法反应转化为高价值产物的铌基催化剂

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Synthesis and Catalytic Applications of Advanced Sn- and Zr-Zeolites Materials.先进的锡和锆沸石材料的合成与催化应用

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Domino reaction catalyzed by zeolites with Brønsted and Lewis acid sites for the production of γ-valerolactone from furfural.

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