Department of Physics, University of Surrey, Guildford, Surrey GU2 7XH, UK.
Phys Med Biol. 2013 Jul 7;58(13):4471-82. doi: 10.1088/0031-9155/58/13/4471. Epub 2013 Jun 13.
Recently, a new family of low-cost x-radiation detectors have been developed, based on semiconducting polymer diodes, which are easy to process, mechanically flexible, relatively inexpensive, and able to cover large areas. To test their potential for radiotherapy applications such as beam monitors or dosimeters, as an alternative to the use of solid-state inorganic detectors, we present the direct detection of 6 MV x-rays from a medical linear accelerator using a thick film, semiconducting polymer detector. The diode was subjected to 4 ms pulses of 6 MV x-rays at a rate of 60 Hz, and produces a linear increase in photocurrent with increasing dose rate (from 16.7 to 66.7 mGy s(-1)). The sensitivity of the diode was found to range from 13 to 20 nC mGy(-1) cm(-3), for operating voltages from -50 to -150 V, respectively. The diode response was found to be stable after exposure to doses up to 15 Gy. Testing beyond this dose range was not carried out. Theoretical calculations show that the addition of heavy metallic nanoparticles to polymer films, even at low volume fractions, increases the x-ray sensitivity of the polymer film/nanoparticle composite so that it exceeds that for silicon over a wide range of x-ray energies. The possibility of detecting x-rays with energies relevant to medical oncology applications opens up the potential for these polymer detectors to be used in detection and imaging applications using medical x-ray beams.
最近,已经开发出了一种基于半导体聚合物二极管的新型低成本 X 射线探测器家族,它们易于加工、机械灵活、相对便宜并且能够覆盖大面积。为了测试它们在放射治疗应用中的潜力,例如束流监视器或剂量计,作为替代使用固态无机探测器,我们使用厚膜半导体聚合物探测器直接检测来自医用线性加速器的 6 MV X 射线。该二极管以 60 Hz 的速率经受 6 MV X 射线的 4 ms 脉冲,并且随着剂量率的增加(从 16.7 到 66.7 mGy s(-1)),光电流呈线性增加。发现二极管的灵敏度范围为 13 至 20 nC mGy(-1) cm(-3),工作电压分别为-50 至-150 V。发现二极管在暴露于高达 15 Gy 的剂量后响应稳定。未进行超过此剂量范围的测试。理论计算表明,即使在低体积分数下,将重金属纳米粒子添加到聚合物膜中也会增加聚合物膜/纳米粒子复合材料的 X 射线灵敏度,使得其在很宽的 X 射线能量范围内超过硅的灵敏度。检测与医学肿瘤学应用相关的 X 射线的可能性为这些聚合物探测器在使用医用 X 射线束的检测和成像应用中开辟了潜力。