NERC Centre for Ecology & Hydrology, Lancaster Environment Centre, Library Av., Bailrigg, Lancaster LA1 4AP, United Kingdom.
J Environ Radioact. 2013 Dec;126:326-37. doi: 10.1016/j.jenvrad.2013.05.005. Epub 2013 Jul 16.
The ICRP and IAEA have recently reported Concentration Ratio values (CRwo-media--equilibrium radionuclide activity concentration in whole organism divided by that in media) for Reference Animals and Plants (RAPs) and a wide range of organism groups, respectively, based on a common online database. Given the large number of data gaps in both publications, there is a need to develop methods for identifying the relative importance of improving currently available CR(wo-media) values. A simple, transparent approach involving the derivation and comparison of predicted internal and external weighted absorbed dose rates for radionuclides considered by ICRP (2009) for terrestrial RAPs is presented. Using the approach of applying a reference value of CR(wo-soil) = 1 or using the maximum reported values where CR(wo-soil) >1, we provisionally identify terrestrial radionuclide RAP combinations which could be considered low priority, notably: Ca, Cr and Ni consistently; Mn for all RAPs except Deer and Pine Tree; and Tc for all RAPs but Wild Grass. Equally, we can systematically identify high priority elements and radioisotopes, which largely, but not exclusively, consist of alpha-emitters (especially isotopes of Ra and Th, but also consistently Am, Cf, Cm, Np, Pa, Po, Pu, U). The analysis highlights the importance of the radiation weighting factor default assumption of 10 for alpha-emitters in the ERICA Tool when comparing the magnitude of the internal dose and trying to identify high priority RAP-isotope combinations. If the unweighted Dose Conversion Coefficient (DCC) values are considered, those for alpha-emitters are often one order of magnitude higher than those due to some beta-gamma emitters for terrestrial RAPs, whereas with the radiation weighting factor applied they are two orders of magnitude higher.
国际辐射防护委员会(ICRP)和国际原子能机构(IAEA)最近根据一个共同的在线数据库,分别报告了参考动物和植物(RAPs)以及广泛的生物体群体的浓度比(CRwo-media--生物体中放射性核素的总活性浓度与介质中的活性浓度之比)值。鉴于这两个出版物中都存在大量的数据差距,因此需要开发方法来确定提高当前可用 CR(wo-media)值的相对重要性。本文提出了一种简单透明的方法,涉及到 ICRP(2009 年)考虑的放射性核素的内部和外部加权吸收剂量率的预测值的推导和比较,用于陆地 RAPs。使用应用 CR(wo-soil)=1 的参考值或使用 CR(wo-soil)>1 时报告的最大值的方法,我们暂时确定了陆地放射性核素 RAP 组合,可以被认为是低优先级的,特别是:Ca、Cr 和 Ni 始终如此;除了鹿和松树之外,所有 RAPs 中的 Mn;除了野生草之外,所有 RAPs 中的 Tc。同样,我们可以系统地确定高优先级的元素和放射性同位素,这些元素和同位素主要但不是完全由α发射体组成(特别是 Ra 和 Th 的同位素,但也包括 Am、Cf、Cm、Np、Pa、Po、Pu、U 的同位素)。该分析强调了在 ERICA 工具中比较内部剂量的大小并试图确定高优先级 RAP-同位素组合时,对α发射体的辐射权重因子默认假设为 10 的重要性。如果考虑未加权的剂量转换系数(DCC)值,则对于陆地 RAPs 的α发射体,这些值通常比某些β-γ发射体高一个数量级,而应用辐射权重因子后,它们则高两个数量级。