1] Advanced Light Source, E. O. Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA [2] Department of Molecular Physics, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, 14195 Berlin, Germany.
Nat Mater. 2013 Oct;12(10):887-92. doi: 10.1038/nmat3717. Epub 2013 Jul 28.
Charge carriers in bilayer graphene are widely believed to be massive Dirac fermions that have a bandgap tunable by a transverse electric field. However, a full transport gap, despite its importance for device applications, has not been clearly observed in gated bilayer graphene, a long-standing puzzle. Moreover, the low-energy electronic structure of bilayer graphene is widely held to be unstable towards symmetry breaking either by structural distortions, such as twist, strain, or electronic interactions that can lead to various ground states. Which effect dominates the physics at low energies is hotly debated. Here we show both by direct band-structure measurements and by calculations that a native imperfection of bilayer graphene, a distribution of twists whose size is as small as ~0.1°, is sufficient to generate a completely new electronic spectrum consisting of massive and massless Dirac fermions. The massless spectrum is robust against strong electric fields, and has a unusual topology in momentum space consisting of closed arcs having an exotic chiral pseudospin texture, which can be tuned by varying the charge density. The discovery of this unusual Dirac spectrum not only complements the framework of massive Dirac fermions, widely relevant to charge transport in bilayer graphene, but also supports the possibility of valley Hall transport.
双层石墨烯中的电荷载流子被广泛认为是具有带隙的相对论性狄拉克费米子,其带隙可以通过横向电场进行调节。然而,尽管对于器件应用至关重要,但在栅控双层石墨烯中,一个完全的传输带隙尚未被清楚地观察到,这是一个长期存在的难题。此外,双层石墨烯的低能电子结构被广泛认为对对称性破坏不稳定,这种破坏可以通过结构扭曲、应变或电子相互作用来实现,从而导致各种基态。在低能区,哪种效应占主导地位一直存在激烈的争论。在这里,我们通过直接能带结构测量和计算表明,双层石墨烯的一个本征缺陷,即大小约为~0.1°的扭曲分布,足以产生一个完全由相对论性狄拉克费米子组成的全新电子能带结构。无质量的能带结构对强电场具有鲁棒性,并且在动量空间中具有不寻常的拓扑结构,由封闭的弧线组成,具有奇特的手性赝自旋纹理,可以通过改变电荷密度来调节。这种异常的狄拉克能带结构的发现不仅补充了广泛应用于双层石墨烯中电荷输运的相对论性狄拉克费米子的框架,而且还支持了谷霍尔输运的可能性。